Optical antenna properties of scanning probe tips: Plasmonic light scattering, tip-sample coupling, and near-field enhancement

被引:86
作者
Behr, Nicolas [1 ]
Raschke, Markus B. [1 ]
机构
[1] Univ Washington, Dept Chem, Seattle, WA 98195 USA
关键词
D O I
10.1021/jp7098009
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The optical near-field distribution and enhancement near the apex of model scanning probe tips are calculated within the quasistatic approximation. The optical tip-sample coupling sensitively depends on both the tip and sample material. This, in addition to the tip-sample distance and apex geometry, is found to affect the spatial resolution that can be obtained in scattering near-field microscopy (s-SNOM). A pronounced structural plasmon resonant behavior is found for gold tips, which redshifts upon tip-sample approach on the length scale given by the tip radius. This near-field tip-sample coupling also allows for surface plasmon excitation in the sample. With the critical dimensions of the tip apex in the range of 10 to several 10s of nanometers, the results are found to be in good agreement with experiment and more rigorous theoretical treatments.
引用
收藏
页码:3766 / 3773
页数:8
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