Interplay of multiple vibrational spectral densities in femtosecond nonlinear spectroscopy of liquids

被引：32

作者：

Khidekel, V

Chernyak, V

Mukamel, S

机构：

[1] Department of Chemistry, University of Rochester, Rochester

来源：

JOURNAL OF CHEMICAL PHYSICS | 1996年 / 105卷 / 19期

关键词：

D O I：

10.1063/1.472639

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The multimode Brownian oscillator model of nonlinear response functions is generalized to include a multielectronic level system Interacting with several spectral densities representing solvent and vibrational coupling to electronic energies, transition dipoles, and permanent dipoles. Applications to resonant and off-resonant transient grating as well as to infrared and fifth-order Raman photon echoes illustrate how the various spectral densities may be probed separately. (C) 1996 American Institute of Physics.

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页码：8543 / 8555

页数：13

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