Multimodel projections of stratospheric ozone in the 21st century

被引:256
作者
Eyring, V. [1 ]
Waugh, D. W.
Bodeker, G. E.
Cordero, E.
Akiyoshi, H.
Austin, J.
Beagley, S. R.
Boville, B. A.
Braesicke, P.
Bruehl, C.
Butchart, N.
Chipperfield, M. P.
Dameris, M.
Deckert, R.
Deushi, M.
Frith, S. M.
Garcia, R. R.
Gettelman, A.
Giorgetta, M. A.
Kinnison, D. E.
Mancini, E.
Manzini, E.
Marsh, D. R.
Matthes, S.
Nagashima, T.
Newman, P. A.
Nielsen, J. E.
Pawson, S.
Pitari, G.
Plummer, D. A.
Rozanov, E.
Schraner, M.
Scinocca, J. F.
Semeniuk, K.
Shepherd, T. G.
Shibata, K.
Steil, B.
Stolarski, R. S.
Tian, W.
Yoshiki, M.
机构
[1] Deutsches Zent Luft & Raunfahrt, Inst Atmospher Phys, Oberpfaffenhofen, Germany
[2] Johns Hopkins Univ, Dept Earth & Planetary Sci, Baltimore, MD 21218 USA
[3] Natl Inst Water & Atmospher Res, Lauder, New Zealand
[4] San Jose State Univ, Dept Meteorol, San Jose, CA 95192 USA
[5] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan
[6] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA
[7] York Univ, Dept Earth & Space Sci & Engn, Toronto, ON M3J 2R7, Canada
[8] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[9] Univ Cambridge, Ctr Atmospher Sci, Cambridge, England
[10] Max Planck Inst Chem, D-55128 Mainz, Germany
[11] Met Off Climate Res Div, Exeter, Devon, England
[12] Univ Leeds, Inst Atmospher Sci, Leeds LS2 9JT, W Yorkshire, England
[13] Meteorol Res Inst, Tsukuba, Ibaraki, Japan
[14] Sci Syst & Applicat Inc, Lanham, MD USA
[15] Max Planck Inst Meteorol, Hamburg, Germany
[16] Univ Aquila, Dipartimento Fis, I-67100 Laquila, Italy
[17] Ist Nazl Geofis & Vulcanol, Ctr Euro Mediterraneo Cambiamenti Climat, Bologna, Italy
[18] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA
[19] Environm Canada, Atomospher Environm Serv, Toronto, ON M3H 5T4, Canada
[20] World Radiat Ctr, Inst Atmospher & Climate Sci ETHZ, Phys Meteorol Observ, Davos, Switzerland
[21] ETH, Inst Atmospher & Climate Sci, Zurich, Switzerland
[22] Univ Victoria, Canadian Ctr Climate Modelling & Anal, Meteorol Serv Canada, Victoria, BC, Canada
[23] Univ Toronto, Dept Phys, Toronto, ON, Canada
基金
英国自然环境研究理事会;
关键词
D O I
10.1029/2006JD008332
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Simulations from eleven coupled chemistry-climate models (CCMs) employing nearly identical forcings have been used to project the evolution of stratospheric ozone throughout the 21st century. The model-to-model agreement in projected temperature trends is good, and all CCMs predict continued, global mean cooling of the stratosphere over the next 5 decades, increasing from around 0.25 K/decade at 50 hPa to around 1 K/decade at 1 hPa under the Intergovernmental Panel on Climate Change ( IPCC) Special Report on Emissions Scenarios (SRES) A1B scenario. In general, the simulated ozone evolution is mainly determined by decreases in halogen concentrations and continued cooling of the global stratosphere due to increases in greenhouse gases (GHGs). Column ozone is projected to increase as stratospheric halogen concentrations return to 1980s levels. Because of ozone increases in the middle and upper stratosphere due to GHG-induced cooling, total ozone averaged over midlatitudes, outside the polar regions, and globally, is projected to increase to 1980 values between 2035 and 2050 and before lowerstratospheric halogen amounts decrease to 1980 values. In the polar regions the CCMs simulate small temperature trends in the first and second half of the 21st century in midwinter. Differences in stratospheric inorganic chlorine (Cl-y) among the CCMs are key to diagnosing the intermodel differences in simulated ozone recovery, in particular in the Antarctic. It is found that there are substantial quantitative differences in the simulated Cly, with the October mean Antarctic Cly peak value varying from less than 2 ppb to over 3.5 ppb in the CCMs, and the date at which the Cly returns to 1980 values varying from before 2030 to after 2050. There is a similar variation in the timing of recovery of Antarctic springtime column ozone back to 1980 values. As most models underestimate peak Cly near 2000, ozone recovery in the Antarctic could occur even later, between 2060 and 2070. In the Arctic the column ozone increase in spring does not follow halogen decreases as closely as in the Antarctic, reaching 1980 values before Arctic halogen amounts decrease to 1980 values and before the Antarctic. None of the CCMs predict future large decreases in the Arctic column ozone. By 2100, total column ozone is projected to be substantially above 1980 values in all regions except in the tropics.
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页数:24
相关论文
共 86 条
[1]   Ozone perturbations in the Arctic summer lower stratosphere as a reflection of NOX chemistry and planetary scale wave activity -: art. no. D03304 [J].
Akiyoshi, H ;
Sugita, T ;
Kanzawa, H ;
Kawamoto, N .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D3)
[2]   Halogen occultation experiment confirmation of stratospheric chlorine decreases in accordance with the Montreal Protocol [J].
Anderson, J ;
Russell, JM ;
Solomon, S ;
Deaver, LE .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D4) :4483-4490
[3]  
[Anonymous], [No title captured]
[4]  
[Anonymous], 50 WMO UNEP
[5]   Uncertainties and assessments of chemistry-climate models of the stratosphere [J].
Austin, J ;
Shindell, D ;
Beagley, SR ;
Brühl, C ;
Dameris, M ;
Manzini, E ;
Nagashima, T ;
Newman, P ;
Pawson, S ;
Pitari, G ;
Rozanov, E ;
Schnadt, C ;
Shepherd, TG .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2003, 3 :1-27
[6]   Evolution of water vapor concentrations and stratospheric age of air in coupled chemistry-climate model simulations [J].
Austin, John ;
Wilson, John ;
Li, Feng ;
Vomel, Holger .
JOURNAL OF THE ATMOSPHERIC SCIENCES, 2007, 64 (03) :905-921
[7]   On the relationship between the strength of the Brewer-Dobson circulation and the age of stratospheric air [J].
Austin, John ;
Li, Feng .
GEOPHYSICAL RESEARCH LETTERS, 2006, 33 (17)
[8]   Ensemble simulations of the decline and recovery of stratospheric ozone [J].
Austin, John ;
Wilson, R. John .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2006, 111 (D16)
[9]   Radiative-dynamical climatology of the first-generation Canadian Middle Atmosphere Model [J].
Beagley, SR ;
deGrandpre, J ;
Koshyk, JN ;
McFarlane, NA ;
Shepherd, TG .
ATMOSPHERE-OCEAN, 1997, 35 (03) :293-331
[10]   Indicators of Antarctic ozone depletion [J].
Bodeker, GE ;
Shiona, H ;
Eskes, H .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2005, 5 :2603-2615