Radial compression and controlled cutting of carbon nanotubes

被引:54
作者
Lordi, V [1 ]
Yao, N [1 ]
机构
[1] Princeton Univ, Princeton Mat Inst, Princeton, NJ 08540 USA
关键词
D O I
10.1063/1.476822
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Utilizing high-resolution transmission electron microscopy, in tandem with molecular dynamics simulations, we conduct a fundamental study of the mechanical force-structure relationship of carbon nanotubes. We study the response of tubes to asymmetrical radial compressive forces, which are directly related to observed structure distortions in HRTEM (high-resolution transmission electron microscopy). We show that the magnitude of such forces can be readily estimated and is related to the shape of the distortion, characterized by percent compression and the radius of the tube, as well as the number of layers for very narrow tubes. The elasticity and resilience of the walls depend on the tube radius and the number of layers. We further suggest that even very large forces produce reversible, elastic distortions, indicating that radial mechanical forces should not be a feasible method to cut a nanotube without causing severe structural damage. (C) 1998 American Institute of Physics.
引用
收藏
页码:2509 / 2512
页数:4
相关论文
共 19 条
[1]   APPLICATION OF A UNIVERSAL FORCE-FIELD TO ORGANIC-MOLECULES [J].
CASEWIT, CJ ;
COLWELL, KS ;
RAPPE, AK .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1992, 114 (25) :10035-10046
[2]   A CARBON NANOTUBE FIELD-EMISSION ELECTRON SOURCE [J].
DEHEER, WA ;
CHATELAIN, A ;
UGARTE, D .
SCIENCE, 1995, 270 (5239) :1179-1180
[3]   Structural flexibility of carbon nanotubes [J].
Iijima, S ;
Brabec, C ;
Maiti, A ;
Bernholc, J .
JOURNAL OF CHEMICAL PHYSICS, 1996, 104 (05) :2089-2092
[4]   HELICAL MICROTUBULES OF GRAPHITIC CARBON [J].
IIJIMA, S .
NATURE, 1991, 354 (6348) :56-58
[5]   Applied physics - Single-molecule transistors [J].
Kouwenhoven, L .
SCIENCE, 1997, 275 (5308) :1896-1897
[6]   STRUCTURAL RIGIDITY AND LOW-FREQUENCY VIBRATIONAL-MODES OF LONG CARBON TUBULES [J].
OVERNEY, G ;
ZHONG, W ;
TOMANEK, D .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1993, 27 (01) :93-96
[7]   UFF, A FULL PERIODIC-TABLE FORCE-FIELD FOR MOLECULAR MECHANICS AND MOLECULAR-DYNAMICS SIMULATIONS [J].
RAPPE, AK ;
CASEWIT, CJ ;
COLWELL, KS ;
GODDARD, WA ;
SKIFF, WM .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1992, 114 (25) :10024-10035
[8]   APPLICATION OF A UNIVERSAL FORCE-FIELD TO METAL-COMPLEXES [J].
RAPPE, AK ;
COLWELL, KS ;
CASEWIT, CJ .
INORGANIC CHEMISTRY, 1993, 32 (16) :3438-3450
[9]   UNRAVELING NANOTUBES - FIELD-EMISSION FROM AN ATOMIC WIRE [J].
RINZLER, AG ;
HAFNER, JH ;
NIKOLAEV, P ;
LOU, L ;
KIM, SG ;
TOMANEK, D ;
NORDLANDER, P ;
COLBERT, DT ;
SMALLEY, RE .
SCIENCE, 1995, 269 (5230) :1550-1553
[10]   ENERGETICS OF NANOSCALE GRAPHITIC TUBULES [J].
ROBERTSON, DH ;
BRENNER, DW ;
MINTMIRE, JW .
PHYSICAL REVIEW B, 1992, 45 (21) :12592-12595