Efficient electrocatalytic oxygen reduction over metal free-nitrogen doped carbon nanocapsules

被引:151
作者
Shanmugam, Sangaraju [1 ]
Osaka, Tetsuya [1 ]
机构
[1] Waseda Univ, Sch Adv Sci & Engn, Tokyo 1698555, Japan
关键词
FUEL-CELL ELECTRODES; CATALYST; NANOTUBES; NANOPARTICLES; ENHANCEMENT; DURABILITY; SUPPORT; ARRAYS;
D O I
10.1039/c1cc10361j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Nitrogen doped carbon nanocapsules (NCNCs) were synthesized as a non-noble electrocatalyst for the ORR using a simple and efficient route. The NCNCs exhibited higher activity than the commercial Pt/C catalyst, excellent stability, and resistance to methanol oxidation in the oxygen reduction reaction.
引用
收藏
页码:4463 / 4465
页数:3
相关论文
共 21 条
[1]   Synthesis, characterization, and manipulation of nitrogen-doped carbon nanotube cups [J].
Allen, Brett L. ;
Kichambare, Padmakar D. ;
Star, Alexander .
ACS NANO, 2008, 2 (09) :1914-1920
[2]   Electrocatalytic reduction of oxygen by FePt alloy nanoparticles [J].
Chen, Wei ;
Kim, Jaemin ;
Sun, Shonheng ;
Chen, Shaowei .
JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (10) :3891-3898
[3]   Nitrogen doped carbon nanotubes and their impact on the oxygen reduction reaction in fuel cells [J].
Chen, Zhu ;
Higgins, Drew ;
Chen, Zhongwei .
CARBON, 2010, 48 (11) :3057-3065
[4]   Nitrogen-Doped Carbon Nanotube Arrays with High Electrocatalytic Activity for Oxygen Reduction [J].
Gong, Kuanping ;
Du, Feng ;
Xia, Zhenhai ;
Durstock, Michael ;
Dai, Liming .
SCIENCE, 2009, 323 (5915) :760-764
[5]   Iron-Based Catalysts with Improved Oxygen Reduction Activity in Polymer Electrolyte Fuel Cells [J].
Lefevre, Michel ;
Proietti, Eric ;
Jaouen, Frederic ;
Dodelet, Jean-Pol .
SCIENCE, 2009, 324 (5923) :71-74
[6]  
Levich V. G., 1962, Physicochemical Hydrodynamics
[7]   Direct Synthesis and Structural Analysis of Nitrogen-Doped Carbon Nanofibers [J].
Lim, Seongyop ;
Yoon, Seong-Ho ;
Mochida, Isao ;
Jung, Doo-Hwan .
LANGMUIR, 2009, 25 (14) :8268-8273
[8]   Development of non-precious metal oxygen-reduction catalysts for PEM fuel cells based on N-doped ordered porous carbon [J].
Liu, Gang ;
Li, Xuguang ;
Ganesan, Prabhu ;
Popov, Branko N. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2009, 93 (1-2) :156-165
[9]   Nitrogen-Doped Ordered Mesoporous Graphitic Arrays with High Electrocatalytic Activity for Oxygen Reduction [J].
Liu, Ruili ;
Wu, Dongqing ;
Feng, Xinliang ;
Muellen, Klaus .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (14) :2565-2569
[10]   Template synthesis and characterization of well-aligned nitrogen containing carbon nanotubes [J].
Maiyalagan, T ;
Viswanathan, B .
MATERIALS CHEMISTRY AND PHYSICS, 2005, 93 (2-3) :291-295