Ground states of a frustrated spin-1/2 antiferromagnet:: Cs2CuCl4 in a magnetic field -: art. no. 214426

We present detailed calculations of the magnetic ground state properties of Cs2CuCl4 in an applied magnetic field, and compare our results with recent experiments. The material is described by a spin Hamiltonian, determined with precision in high field measurements, in which the main interaction is antiferromagnetic Heisenberg exchange between neighboring spins on an anisotropic triangular lattice. An additional, weak Dzyaloshinskii-Moriya interaction introduces easy-plane anisotropy, so that behavior is different for transverse and longitudinal field directions. We determine the phase diagram as a function of field strength for both field directions at zero temperature, using a classical approximation as a first step. Building on this, we calculate the effect of quantum fluctuations on the ordering wave vector and components of the ordered moments, using both linear spinwave theory and a mapping to a Bose gas which gives exact results when the magnetization is almost saturated. Many aspects of the experimental data are well accounted for by this approach.