Ostwald ripening of two-dimensional islands on Si(001)

被引:193
作者
Bartelt, NC [1 ]
Theis, W [1 ]
Tromp, RM [1 ]
机构
[1] IBM CORP, DIV RES, THOMAS J WATSON RES CTR, YORKTOWN HTS, NY 10598 USA
来源
PHYSICAL REVIEW B | 1996年 / 54卷 / 16期
关键词
D O I
10.1103/PhysRevB.54.11741
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have used low-energy electron microscopy to study two-dimensional island ripening on Si(001). By studying the behavior of individual islands compared to their surroundings, we are able to quantify the step-edge attachment and terrace diffusion processes that are responsible for the ripening. By comparing the time dependence of specific configurations of islands to simulations, we find correlations in the rate of change of an island's area with the sizes of neighboring islands, implying that the chemical potential of the adatom sea is not uniform as classical theories of Ostwald ripening assume. From measurements of the time dependence of each island, we chart out these nonuniformities and relate them to adatom diffusion coefficients.
引用
收藏
页码:11741 / 11751
页数:11
相关论文
共 37 条
[1]   Low-energy electron microscopy study of step mobilities on Si(001) [J].
Bartelt, NC ;
Tromp, RM .
PHYSICAL REVIEW B, 1996, 54 (16) :11731-11740
[2]   STEP CAPILLARY WAVES AND EQUILIBRIUM ISLAND SHAPES ON SI(001) [J].
BARTELT, NC ;
TROMP, RM ;
WILLIAMS, ED .
PHYSICAL REVIEW LETTERS, 1994, 73 (12) :1656-1659
[3]   THE EQUILIBRATION OF TERRACE WIDTH DISTRIBUTIONS ON STEPPED SURFACES [J].
BARTELT, NC ;
GOLDBERG, JL ;
EINSTEIN, TL ;
WILLIAMS, ED .
SURFACE SCIENCE, 1992, 273 (1-2) :252-260
[4]   MEASURING SURFACE MASS DIFFUSION-COEFFICIENTS BY OBSERVING STEP FLUCTUATIONS [J].
BARTELT, NC ;
EINSTEIN, TL ;
WILLIAMS, ED .
SURFACE SCIENCE, 1994, 312 (03) :411-421
[5]   BROWNIAN-MOTION OF STEPS ON SI(111) [J].
BARTELT, NC ;
GOLDBERG, JL ;
EINSTEIN, TL ;
WILLIAMS, ED ;
HEYRAUD, JC ;
METOIS, JJ .
PHYSICAL REVIEW B, 1993, 48 (20) :15453-15456
[6]   THEORY OF OSTWALD RIPENING FOR OPEN SYSTEMS [J].
BEENAKKER, CWJ ;
ROSS, J .
JOURNAL OF CHEMICAL PHYSICS, 1985, 83 (09) :4710-4714
[7]  
Bevington R., 1969, DATA REDUCTION ERROR
[8]   DEPENDENCE OF OSTWALD RIPENING KINETICS ON PARTICLE-VOLUME FRACTION [J].
BRAILSFORD, AD ;
WYNBLATT, P .
ACTA METALLURGICA, 1979, 27 (03) :489-497
[9]   CLUSTERING ACROSS CONCENTRATION GRADIENTS [J].
CARLOW, GR ;
ZINKEALLMANG, M .
CANADIAN JOURNAL OF PHYSICS, 1994, 72 (11-12) :812-817
[10]  
CHAKRAVE.BK, 1967, J PHYS CHEM SOLIDS, V28, P2401, DOI 10.1016/0022-3697(67)90026-1