Recent Changes in Particulate Air Pollution over China Observed from Space and the Ground: Effectiveness of Emission Control

被引:110
作者
Lin, Jintai [1 ,2 ,3 ]
Nielsen, Chris P. [2 ,3 ]
Zhao, Yu [2 ,3 ]
Lei, Yu [2 ,3 ]
Liu, Yang [4 ]
Mcelroy, Michael B. [2 ,3 ]
机构
[1] Peking Univ, Dept Atmospher & Ocean Sci, Sch Phys, Beijing 100871, Peoples R China
[2] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[3] Harvard Univ, Harvard China Project, Cambridge, MA 02138 USA
[4] Emory Univ, Rollins Sch Publ Hlth, Dept Environm & Occupat Hlth, Atlanta, GA 30322 USA
基金
中国国家自然科学基金; 美国国家科学基金会;
关键词
AEROSOL OPTICAL-THICKNESS; TROPOSPHERIC NO2; INTEX-B; SATELLITE; IMPACT; OZONE; ASIA; OMI;
D O I
10.1021/es101094t
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The Chinese government has moved aggressively since 2005 to reduce emissions of a number of pollutants including primary particulate matter (PM) and sulfur dioxide (SO2), efforts inadvertently aided since late 2008 by economic recession. Satellite observations of aerosol optical depth (AOD) and column nitrogen dioxide (NO2) provide independent indicators of emission trends, clearly reflecting the sharp onset of the recession in the fall of 2008 and rebound of the economy in the latter half of 2009. Comparison of ADD with ground-based observations of PM over a longer period indicate that emission-control policies have not been successful in reducing concentrations of aerosol pollutants at smaller size range over industrialized regions of China. The lack of success is attributed to the increasing importance of anthropogenic secondary aerosols formed from precursor species including nitrogen oxides (NOx), non-methane volatile organic compounds (NMVOC), and ammonia (NH3).
引用
收藏
页码:7771 / 7776
页数:6
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