Effective schemes to control the dynamic behavior of the water transport in the membrane of PEM fuel cell

被引:37
作者
Chen, FL [1 ]
Chu, HS
Soong, CY
Yan, WM
机构
[1] Natl Taiwan Univ, Inst Appl Mech, Taipei 106, Taiwan
[2] Ind Technol Res Inst, Energy Resources Lab, Hsinchu 310, Taiwan
[3] Feng Chia Univ, Dept Aerosp & Syst Engn, Taichung 40724, Taiwan
[4] Huafan Univ, Dept Mechatron Engn, Taipei 22305, Taiwan
关键词
PEM fuel cell; membrane; water management; transient behavior; dynamic response time;
D O I
10.1016/j.jpowsour.2004.08.026
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We have investigated the transient behavior of the water transport across the membrane of the PEM fuel cell to seek- for effective control schemes so that the best dynamic performance of the fuel cell can be obtained. It is found that both a larger starting operational current density i(0) and a smaller operational current density i can lead to a smaller dynamic response time t(ss), the time for the water distribution across the membrane to reach the steady state. Present results nevertheless point out that the most powerful as well as the most feasible control scheme. is to control the humidification parameter k, i.e. to adjust the water content of the feeding fuel. so that the t(ss) would remain steadily in a reasonably low value in a wide range of water flux fraction beta, another control parameter of the membrane. The present conclusion can be useful for the design of the PEM fuel cell when its application on the dynamic mobile system is concerned. (C) 2004 Elsevier B.V. All rights reserved.
引用
收藏
页码:243 / 249
页数:7
相关论文
共 23 条
[1]   A MATHEMATICAL-MODEL OF THE SOLID-POLYMER-ELECTROLYTE FUEL-CELL [J].
BERNARDI, DM ;
VERBRUGGE, MW .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1992, 139 (09) :2477-2491
[2]   WATER-BALANCE CALCULATIONS FOR SOLID-POLYMER-ELECTROLYTE FUEL-CELLS [J].
BERNARDI, DM .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1990, 137 (11) :3344-3350
[3]  
BERNARDI DM, 1991, AICHE J, V37, P151
[4]   Three-dimensional computational analysis of transport phenomena in a PEM fuel cell [J].
Berning, T ;
Lu, DM ;
Djilali, N .
JOURNAL OF POWER SOURCES, 2002, 106 (1-2) :284-294
[5]  
CHEN F, 2003, IN PRESS J ELECTROAN
[6]   Quantum jumps in the PEMFC science and technology from the 1960s to the year 2000 Part I. Fundamental scientific aspects [J].
Costamagna, P ;
Srinivasan, S .
JOURNAL OF POWER SOURCES, 2001, 102 (1-2) :242-252
[7]   Quantum jumps in the PEMFC science and technology from the 1960s to the year 2000 Part II. Engineering, technology development and application aspects [J].
Costamagna, P ;
Srinivasan, S .
JOURNAL OF POWER SOURCES, 2001, 102 (1-2) :253-269
[8]   Influence of heat transfer on gas and water transport in fuel cells [J].
Djilali, N ;
Lu, DM .
INTERNATIONAL JOURNAL OF THERMAL SCIENCES, 2002, 41 (01) :29-40
[9]   WATER AND THERMAL MANAGEMENT IN SOLID-POLYMER-ELECTROLYTE FUEL-CELLS [J].
FULLER, TF ;
NEWMAN, J .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1993, 140 (05) :1218-1225
[10]   Development and application of a generalised steady-state electrochemical model for a PEM fuel cell [J].
Mann, RF ;
Amphlett, JC ;
Hooper, MAI ;
Jensen, HM ;
Peppley, BA ;
Roberge, PR .
JOURNAL OF POWER SOURCES, 2000, 86 (1-2) :173-180