High harmonic generation spectra of neutral helium by the complex-scaled (t,t') method: Role of dynamical electron correlation

被引:56
作者
Moiseyev, N
Weinhold, F
机构
[1] TECHNION ISRAEL INST TECHNOL,MINERVA CTR NONLINEAR PHYS COMPLEX SYST,IL-32000 HAIFA,ISRAEL
[2] UNIV WISCONSIN,INST THEORET CHEM,MADISON,WI 53706
[3] UNIV WISCONSIN,DEPT CHEM,MADISON,WI 53706
关键词
D O I
10.1103/PhysRevLett.78.2100
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Using highly correlated Hylleraas-type wave functions of S-1 and P-1 symmetry, we show how the harmonic generation spectrum of 1(1)S He (including short wavelength members previously attributed to He+) arise from a radial-angular ''descreening'' mechanism, This provides the first indication that harmonic generation spectrum can arise from strong dynamical electron correlations rather than purely as a ''one-electron phenomenon.''
引用
收藏
页码:2100 / 2103
页数:4
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