Photoemission spectra of deuterated silicon clusters:: experiment and theory

被引：12

作者：

Kronik, L

Fromherz, R

Ko, E

Ganteför, G

Chelikowsky, JR

机构：

[1] Univ Minnesota, Minnesota Supercomp Inst, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA

[2] Univ Konstanz, Dept Phys, D-78457 Constance, Germany

来源：

EUROPEAN PHYSICAL JOURNAL D | 2003年 / 24卷 / 1-3期

关键词：

D O I：

10.1140/epjd/e2003-00186-5

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We compare experimentally measured and ab initio computed photoelectron spectra of negatively charged deuterated silicon clusters (SimDn-, 4 less than or equal to m less than or equal to 10, 0 less than or equal to n less than or equal to 2) produced in a plasma environment. Based on this comparison, we discuss the kinetics and thermodynamics of the cluster formation and the effect of deuterium on the geometrical and electronic structure of the clusters.

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页码：33 / 36

页数：4

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