A photoelectrochemical device for visible light driven water splitting by a molecular ruthenium catalyst assembled on dye-sensitized nanostructured TiO2

被引:210
作者
Li, Lin [1 ]
Duan, Lele [1 ]
Xu, Yunhua [1 ]
Gorlov, Mikhail [1 ]
Hagfeldt, Anders [1 ,2 ]
Sun, Licheng [1 ,3 ]
机构
[1] Royal Inst Technol, Ctr Mol Devices, Dept Chem, Sch Chem Sci & Engn, S-10044 Stockholm, Sweden
[2] Uppsala Univ, Dept Phys & Analyt Chem, S-75105 Uppsala, Sweden
[3] Dalian Univ Technol, DUT KTH Joint Educ & Res Ctr Mol Devices, State Key Lab Fine Chem, Dalian 116012, Peoples R China
基金
瑞典研究理事会;
关键词
OXIDATION CATALYST; ARTIFICIAL PHOTOSYNTHESIS; POLYMER MEMBRANE; COMPLEX;
D O I
10.1039/c0cc01828g
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A photoelectrochemical device with a molecular Ru catalyst assembled via pH-modified Nafion on a dye-sensitized nanostructured TiO2 film as anode and a Pt foil as cathode has been successfully demonstrated to split water into O-2 and H-2 driven by visible light.
引用
收藏
页码:7307 / 7309
页数:3
相关论文
共 22 条
[1]  
Brimblecombe R, 2008, ANGEW CHEM, V120, P7445
[2]   Solar Driven Water Oxidation by a Bioinspired Manganese Molecular Catalyst [J].
Brimblecombe, Robin ;
Koo, Annette ;
Dismukes, G. Charles ;
Swiegers, Gerhard F. ;
Spiccia, Leone .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (09) :2892-+
[3]   Molecular water-oxidation catalysts for photoelectrochemical cells [J].
Brimblecombe, Robin ;
Dismukes, G. Charles ;
Swiegers, Gerhard F. ;
Spiccia, Leone .
DALTON TRANSACTIONS, 2009, (43) :9374-9384
[4]   Sustained Water Oxidation by [Mn4O4]7+ Core Complexes Inspired by Oxygenic Photosynthesis [J].
Brimblecombe, Robin ;
Kolling, Derrick R. J. ;
Bond, Alan M. ;
Dismukes, G. Charles ;
Swiegers, Gerhard F. ;
Spiccia, Leone .
INORGANIC CHEMISTRY, 2009, 48 (15) :7269-7279
[5]   Development of Bioinspired Mn4O4-Cubane Water Oxidation Catalysts: Lessons from Photosynthesis [J].
Dismukes, G. Charles ;
Brimblecombe, Robin ;
Felton, Greg A. N. ;
Pryadun, Ruslan S. ;
Sheats, John E. ;
Spiccia, Leone ;
Swiegers, Gerhard F. .
ACCOUNTS OF CHEMICAL RESEARCH, 2009, 42 (12) :1935-1943
[6]   Visible Light-Driven Water Oxidation by a Molecular Ruthenium Catalyst in Homogeneous System [J].
Duan, Lele ;
Xu, Yunhua ;
Zhang, Pan ;
Wang, Mei ;
Sun, Licheng .
INORGANIC CHEMISTRY, 2010, 49 (01) :209-215
[7]   Isolated Seven-Coordinate Ru(IV) Dimer Complex with [HOHOH]- Bridging Ligand as an Intermediate for Catalytic Water Oxidation [J].
Duan, Lele ;
Fischer, Andreas ;
Xu, Yunhua ;
Sun, Licheng .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (30) :10397-+
[8]   ELECTROCHEMICAL PHOTOLYSIS OF WATER AT A SEMICONDUCTOR ELECTRODE [J].
FUJISHIMA, A ;
HONDA, K .
NATURE, 1972, 238 (5358) :37-+
[9]   Phosphonate-based bipyridine dyes for stable photovoltaic devices [J].
Gillaizeau-Gauthier, I ;
Odobel, F ;
Alebbi, M ;
Argazzi, R ;
Costa, E ;
Bignozzi, CA ;
Qu, P ;
Meyer, GJ .
INORGANIC CHEMISTRY, 2001, 40 (23) :6073-6079
[10]   Photoelectrochemical cells [J].
Grätzel, M .
NATURE, 2001, 414 (6861) :338-344