Unbroken Perovskite: Interplay of Morphology, Electro-optical Properties, and Ionic Movement

被引:252
作者
Correa-Baena, Juan-Pablo [1 ]
Anaya, Miguel [2 ]
Lozano, Gabriel [2 ]
Tress, Wolfgang [3 ]
Domanski, Konrad [3 ]
Saliba, Michael [3 ]
Matsui, Taisuke [4 ]
Jacobsson, Tor Jesper [1 ]
Calvo, Mauricio E. [2 ]
Abate, Antonio [3 ,5 ]
Gratzel, Michael [3 ]
Miguez, Hernan [2 ]
Hagfeldt, Anders [1 ]
机构
[1] Ecole Polytech Fed Lausanne, Inst Chem Sci & Engn, Lab Photomol Sci, CH-1015 Lausanne, Switzerland
[2] Univ Seville, Spanish Natl Res Council, Inst Mat Sci Seville, Ave Americo Vespucio 49, Seville 41092, Spain
[3] Ecole Polytech Fed Lausanne, Inst Chem Sci & Engn, Lab Photon & Interfaces, CH-1015 Lausanne, Switzerland
[4] Panasonic Corp, Div Res, 1006 Oaza Kadoma, Kadoma, Osaka 5718501, Japan
[5] Univ Fribourg, Adolphe Merkle Inst, Ch Musee 3, CH-1700 Fribourg, Switzerland
基金
欧洲研究理事会;
关键词
SOLAR-CELLS; CHARGE-TRANSPORT; MESOPOROUS TIO2; HYSTERESIS; DOPANTS; LENGTHS; LAYERS;
D O I
10.1002/adma.201600624
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Hybrid organic-inorganic perovskite materials have risen up as leading components for light-harvesting applications. However, to date many questions are still open concerning the operation of perovskite solar cells (PSCs). A systematic analysis of the interplay among structural features, optoelectronic performance, and ionic movement behavior for FA(0.83)MA(0.17)Pb(I0.83Br0.17)(3) PSCs is presented, which yield high power conversion efficiencies up to 20.8%.
引用
收藏
页码:5031 / 5037
页数:7
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