Strongly coverage-dependent excitations of adsorbed molecular hydrogen
被引:59
作者:
Gupta, JA
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机构:
IBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USAIBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USA
Gupta, JA
[1
]
Lutz, CP
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IBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USAIBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USA
Lutz, CP
[1
]
Heinrich, AJ
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h-index: 0
机构:
IBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USAIBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USA
Heinrich, AJ
[1
]
Eigler, DM
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机构:
IBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USAIBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USA
Eigler, DM
[1
]
机构:
[1] IBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USA
来源:
PHYSICAL REVIEW B
|
2005年
/
71卷
/
11期
关键词:
D O I:
10.1103/PhysRevB.71.115416
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
We have observed prominent nonlinearities in differential conductance spectra of H-2 on copper surfaces using a low-temperature scanning tunneling microscope. These nonlinearities result from transitions between states of H-2 with distinct conductances. Tunneling electrons drive these transitions by giving up energy to highly coverage-dependent excitations that do not correspond to known vibrational or rotational modes of H-2. The nonlinear conductance features can be modeled by extending the conventional framework for inelastic electron tunneling spectroscopy to include saturation effects.