Tracing biomass burning plumes from the Southern Hemisphere during the AMMA 2006 wet season experiment

被引:60
作者
Mari, C. H. [1 ]
Cailley, G. [2 ]
Corre, L. [1 ]
Saunois, M. [1 ]
Attie, J. L. [1 ]
Thouret, V. [1 ]
Stohl, A. [3 ]
机构
[1] Univ Toulouse, CNRS, INSU, Lab Aerol, Toulouse, France
[2] SILOGIC, Toulouse, France
[3] Norwegian Inst Air Res, Kjeller, Norway
关键词
D O I
10.5194/acp-8-3951-2008
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The Lagrangian particle dispersion model FLEXPART coupled with daily active fire products provided by the MODIS instrument was used to forecast the intrusions of the southern hemispheric fire plumes in the Northern Hemisphere during the AMMA (African Monsoon Multidisciplinary Analysis) fourth airborne campaign from 25 July to 31 August 2006 (Special Operation Period SOP2-a2). The imprint of the biomass burning plumes over the Gulf of Guinea showed a well marked intraseasonal variability which is controlled by the position and strength of the southern hemispheric African Easterly Jet (AEJ-S). Three different periods were identified which correspond to active and break phases of the AEJ-S: 25 July-2 August (active phase), 3 August-8 August (break phase) and 9 August-31 August (active phase). During the AEJ-S active phases, the advection of the biomass burning plumes out over the Atlantic ocean was efficient in the mid-troposphere. During the AEJ-S break phases, pollutants emitted by fires were trapped over the continent where they accumulated. The continental circulation increased the possibility for the biomass burning plumes to reach the convective regions located further north. As a consequence, biomass burning plumes were found in the upper troposphere over the Gulf of Guinea during the AEJ-S break phase. Observational evidences from the ozonesounding network at Cotonou and the carbon monoxide measured by MOPITT confirmed the alternation of the AEJ-S phases with low ozone and CO in the mid-troposphere over the Gulf of Guinea during the break phase.
引用
收藏
页码:3951 / 3961
页数:11
相关论文
共 80 条
[1]   The influence of African air pollution on regional and global tropospheric ozone [J].
Aghedo, A. M. ;
Schultz, M. G. ;
Rast, S. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 :1193-1212
[2]   Smoking rain clouds over the Amazon [J].
Andreae, MO ;
Rosenfeld, D ;
Artaxo, P ;
Costa, AA ;
Frank, GP ;
Longo, KM ;
Silva-Dias, MAF .
SCIENCE, 2004, 303 (5662) :1337-1342
[3]   Emission of trace gases and aerosols from biomass burning [J].
Andreae, MO ;
Merlet, P .
GLOBAL BIOGEOCHEMICAL CYCLES, 2001, 15 (04) :955-966
[4]   A meteorological overview of the TRACE a period [J].
Bachmeier, AS ;
Fuelberg, HE .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D19) :23881-23888
[5]  
BURPEE RW, 1972, J ATMOS SCI, V29, P77, DOI 10.1175/1520-0469(1972)029<0077:TOASOE>2.0.CO
[6]  
2
[7]   Diurnal cycle of dust and cirrus over West Africa as seen from Meteosat Second Generation satellite and a regional forecast model [J].
Chaboureau, Jean-Pierre ;
Tulet, Pierre ;
Mari, Celine .
GEOPHYSICAL RESEARCH LETTERS, 2007, 34 (02)
[8]   The subtropical global plume in the Pacific Exploratory Mission-Tropics A (PEM-Tropics A), PEM-Tropics B, and the Global Atmospheric Sampling Program (GASP): How tropical emissions affect the remote Pacific [J].
Chatfield, RB ;
Guo, Z ;
Sachse, GW ;
Blake, DR ;
Blake, NJ .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D16)
[9]   A general model of how fire emissions and chemistry produce African/oceanic plumes (O-3, CO, PAN, smoke) in TRACE A [J].
Chatfield, RB ;
Vastano, JA ;
Singh, HB ;
Sachse, G .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D19) :24279-24306
[10]   BIOMASS BURNING IN THE TROPICS - IMPACT ON ATMOSPHERIC CHEMISTRY AND BIOGEOCHEMICAL CYCLES [J].
CRUTZEN, PJ ;
ANDREAE, MO .
SCIENCE, 1990, 250 (4988) :1669-1678