Plasmonic modes of annular nanoresonators imaged by spectrally resolved cathodoluminescence

被引:61
作者
Hofmann, Carrie E. [1 ]
Vesseur, Ernst Jan R. [2 ]
Sweatlock, Luke A. [1 ]
Lezec, Henri J. [1 ,3 ]
Garcia de Abajo, F. Javier [4 ]
Polman, Albert [1 ,2 ]
Atwater, Harry A. [1 ,2 ]
机构
[1] CALTECH, Thomas J Watson Lab Appl Phys, Pasadena, CA 91125 USA
[2] FOM, Inst Atom & Mol Phys, Ctr Nanophoton, NL-1098 SJ Amsterdam, Netherlands
[3] Ctr Natl Rech Sci, F-75794 Paris 16, France
[4] CSIC, Inst Opt, Madrid 28006, Spain
关键词
D O I
10.1021/nl071789f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report the observation of plasmonic modes of annular resonators in nanofabricated Ag and Au surfaces that are imaged by spectrally resolved cathodoluminescence. A highly focused 30 keV electron beam is used to excite localized surface plasmons that couple to collective resonant modes of the nanoresonators. We demonstrate unprecedented resolution of plasmonic mode excitation and by combining these observations with full-field simulations find that cathodoluminescence in plasmonic nanostructures is most efficiently excited at positions corresponding to antinodes in the modal electric field intensity.
引用
收藏
页码:3612 / 3617
页数:6
相关论文
共 29 条
[1]   Surface plasmon subwavelength optics [J].
Barnes, WL ;
Dereux, A ;
Ebbesen, TW .
NATURE, 2003, 424 (6950) :824-830
[2]   Generation of traveling surface plasmon waves by free-electron impact [J].
Bashevoy, M. V. ;
Jonsson, F. ;
Krasavin, A. V. ;
Zheludev, N. I. ;
Chen, Y. ;
Stockman, M. I. .
NANO LETTERS, 2006, 6 (06) :1113-1115
[3]   Surface plasmon amplification by stimulated emission of radiation: Quantum generation of coherent surface plasmons in nanosystems [J].
Bergman, DJ ;
Stockman, MI .
PHYSICAL REVIEW LETTERS, 2003, 90 (02) :4
[4]   Mapping surface plasmons at the nanometre scale with an electron beam [J].
Bosman, Michel ;
Keast, Vicki J. ;
Watanabe, Masashi ;
Maaroof, Abbas I. ;
Cortie, Michael B. .
NANOTECHNOLOGY, 2007, 18 (16)
[5]   Channel plasmon subwavelength waveguide components including interferometers and ring resonators [J].
Bozhevolnyi, SI ;
Volkov, VS ;
Devaux, E ;
Laluet, JY ;
Ebbesen, TW .
NATURE, 2006, 440 (7083) :508-511
[6]   Experimental analysis of surface plasmon behavior in metallic circular slits [J].
Chang, Chin-Kai ;
Lin, Ding-Zheng ;
Yeh, Chau-Shioung ;
Lee, Chih-Kung ;
Chang, Yu-Chia ;
Lin, Ming-Wei ;
Yeh, Ji-Tian ;
Liu, Jung-Ming .
APPLIED PHYSICS LETTERS, 2007, 90 (06)
[7]  
*CST, 2000, MAXW EQ FIN INT ALG
[8]  
de Abajo FJG, 1998, PHYS REV LETT, V80, P5180
[9]   Retarded field calculation of electron energy loss in inhomogeneous dielectrics [J].
de Abajo, FJG ;
Howie, A .
PHYSICAL REVIEW B, 2002, 65 (11) :1154181-11541817
[10]   Planar metal plasmon waveguides: frequency-dependent dispersion, propagation, localization, and loss beyond the free electron model [J].
Dionne, JA ;
Sweatlock, LA ;
Atwater, HA ;
Polman, A .
PHYSICAL REVIEW B, 2005, 72 (07)