Selective local nitrogen doping in a TiO2 electrode for enhancing photoelectrochemical water splitting

被引:38
作者
Cao, Junyu [1 ]
Zhang, Yuanjian [2 ]
Tong, Hua [1 ,3 ]
Li, Peng [1 ,2 ,4 ]
Kako, Tetsuya [1 ]
Ye, Jinhua [1 ,2 ,3 ,4 ]
机构
[1] Natl Inst Mat Sci, Catalyt Mat Grp, Environm Remediat Mat Unit, Tsukuba, Ibaraki, Japan
[2] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton WPI MANA, Tsukuba, Ibaraki, Japan
[3] Tianjin Univ, Sch Mat Sci & Engn, TU NIMS Joint Res Ctr, Tianjin 300072, Peoples R China
[4] Hokkaido Univ, Grad Sch Sci, Dept Chem, Sapporo, Hokkaido, Japan
关键词
VISIBLE-LIGHT IRRADIATION; DOPED TITANIUM-DIOXIDE; THIN-FILMS; ALPHA-FE2O3; PHOTOELECTRODES; HYDROGEN GENERATION; SEMICONDUCTOR; PHOTOCATALYSIS; PHOTOOXIDATION; PHOTOLYSIS; CRYSTAL;
D O I
10.1039/c2cc33662f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Selective local N-doped TiO2 electrodes were fabricated using a pulsed laser deposition method. Different from the uniform nitrogen-doping in TiO2 electrodes showing the diminution of IPCE in the UV light region, the inner nitrogen-doped TiO2 electrode uniquely enhanced IPCE in the UV light region significantly (up to 95% at 320 nm, 1.23 V vs. SHE).
引用
收藏
页码:8649 / 8651
页数:3
相关论文
共 25 条
[1]   Metal oxide photoelectrodes for hydrogen generation using solar radiation-driven water splitting [J].
Aroutiounian, VM ;
Arakelyan, VM ;
Shahnazaryan, GE .
SOLAR ENERGY, 2005, 78 (05) :581-592
[2]   ELECTROCHEMICAL PHOTOLYSIS OF WATER AT A SEMICONDUCTOR ELECTRODE [J].
FUJISHIMA, A ;
HONDA, K .
NATURE, 1972, 238 (5358) :37-+
[3]   Photoelectrochemical cells [J].
Grätzel, M .
NATURE, 2001, 414 (6861) :338-344
[4]   ENVIRONMENTAL APPLICATIONS OF SEMICONDUCTOR PHOTOCATALYSIS [J].
HOFFMANN, MR ;
MARTIN, ST ;
CHOI, WY ;
BAHNEMANN, DW .
CHEMICAL REVIEWS, 1995, 95 (01) :69-96
[5]   HIGHLY EFFICIENT SEMICONDUCTING TIO2 PHOTOELECTRODES PREPARED BY AEROSOL PYROLYSIS [J].
KAVAN, L ;
GRATZEL, M .
ELECTROCHIMICA ACTA, 1995, 40 (05) :643-652
[6]   Rutile and anatase mixed crystal TiO2 thin films prepared by pulsed laser deposition [J].
Kitazawa, Sin-iti ;
Choi, Yeongzoo ;
Yamamoto, Shunya ;
Yamaki, Tetsuya .
THIN SOLID FILMS, 2006, 515 (04) :1901-1904
[7]   Electrodeposited Aluminum-Doped α-Fe2O3 Photoelectrodes: Experiment and Theory [J].
Kleiman-Shwarsctein, Alan ;
Huda, Muhammad N. ;
Walsh, Aron ;
Yan, Yanfa ;
Stucky, Galen D. ;
Hu, Yong-Sheng ;
Al-Jassim, Mowafak M. ;
McFarland, Eric W. .
CHEMISTRY OF MATERIALS, 2010, 22 (02) :510-517
[8]   Structural, electrical, optical, and photoelectrochemical properties of thin titanium oxinitride films (TiO2-2xNx with 0≤x≤1) [J].
Koslowski, U. ;
Ellmer, K. ;
Bogdanoff, P. ;
Dittrich, T. ;
Guminskaya, T. ;
Tributsch, H. .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A, 2006, 24 (06) :2199-2205
[9]   Spray pyrolytically deposited nanoporous Ti4+ doped hematite thin films for efficient photoelectrochemical splitting of water [J].
Kumari, Saroj ;
Singh, Aadesh P. ;
Sonal ;
Deva, Dinesh ;
Shrivastav, Rohit ;
Dass, Sahab ;
Satsangi, Vibha R. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2010, 35 (09) :3985-3990
[10]   Photocatalytic activity of pulsed laser deposited TiO2 thin films [J].
Lin, H. ;
Rumaiz, Abdul K. ;
Schulz, Meghan ;
Wang, Demin ;
Rock, Reza ;
Huang, C. P. ;
Shah, S. Ismat .
MATERIALS SCIENCE AND ENGINEERING B-ADVANCED FUNCTIONAL SOLID-STATE MATERIALS, 2008, 151 (02) :133-139