Model of defect diffusion and development of the boson peak in an amorphous solid

被引:25
作者
Das, SP [1 ]
机构
[1] Jawaharlal Nehru Univ, Sch Phys Sci, New Delhi 110067, India
[2] Hahn Meitner Inst Berlin GmbH, D-14109 Berlin, Germany
关键词
D O I
10.1103/PhysRevE.59.3870
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
A schematic model is proposed for understanding the boson peak as a consequence of the coupling between slowly decaying density fluctuations and the transverse sound modes th;lt develop in the amorphous solid. The present analysis demonstrates that the nature of the dynamics of defect densities in the disordered system plays a crucial role for the appearance of the peak. We compare the results for the dynamic structure factor with the scattering data of Sokolov et al.. [J. Non-Cryst. Solids 172-174. 138 (1994)]. With the relaxation time for the defects becoming longer which is the case more appropriate for the strong glasses as compared to the fragile glasses where structural degradation occurs more easily, the boson peak become more pronounced.
引用
收藏
页码:3870 / 3875
页数:6
相关论文
共 34 条
[1]   LOW-FREQUENCY RAMAN-SPECTROSCOPY OF SUPERCOOLED FRAGILE LIQUIDS ANALYZED WITH SCHEMATIC MODE-COUPLING MODELS [J].
ALBASIMIONESCO, C ;
KRAUZMAN, M .
JOURNAL OF CHEMICAL PHYSICS, 1995, 102 (16) :6574-6585
[2]   RELAXATION IN LIQUIDS, POLYMERS AND PLASTIC CRYSTALS - STRONG FRAGILE PATTERNS AND PROBLEMS [J].
ANGELL, CA .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 1991, 131 :13-31
[3]   DYNAMICS OF SUPERCOOLED LIQUIDS AND THE GLASS-TRANSITION [J].
BENGTZELIUS, U ;
GOTZE, W ;
SJOLANDER, A .
JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 1984, 17 (33) :5915-5934
[4]   HYDRODYNAMICS OF AMORPHOUS SOLIDS WITH APPLICATION TO LIGHT-SCATTERING SPECTRUM [J].
COHEN, C ;
FLEMING, PD ;
GIBBS, JH .
PHYSICAL REVIEW B, 1976, 13 (02) :866-877
[5]   LIQUID-GLASS TRANSITION, A FREE-VOLUME APPROACH [J].
COHEN, MH ;
GREST, GS .
PHYSICAL REVIEW B, 1979, 20 (03) :1077-1098
[6]   FLUCTUATING NONLINEAR HYDRODYNAMICS AND THE LIQUID-GLASS TRANSITION [J].
DAS, SP ;
MAZENKO, GF .
PHYSICAL REVIEW A, 1986, 34 (03) :2265-2282
[7]   HYDRODYNAMIC THEORY OF THE GLASS-TRANSITION [J].
DAS, SP ;
MAZENKO, GF ;
RAMASWAMY, S ;
TONER, JJ .
PHYSICAL REVIEW LETTERS, 1985, 54 (02) :118-121
[8]   FLUCTUATING HYDRODYNAMICS AND DIFFUSION IN AMORPHOUS SOLIDS [J].
DAS, SP ;
SCHILLING, R .
PHYSICAL REVIEW E, 1994, 50 (02) :1265-1273
[9]   LIGHT-SCATTERING AND DIELECTRIC STUDIES ON GLASS-FORMING LIQUIDS [J].
FISCHER, EW .
PHYSICA A, 1993, 201 (1-3) :183-206
[10]   HYDRODYNAMICS OF SOLIDS [J].
FLEMING, PD ;
COHEN, C .
PHYSICAL REVIEW B, 1976, 13 (02) :500-516