Preventing Graphene Sheets from Restacking for High-Capacitance Performance

被引:338
作者
Wang, Yan [1 ]
Wu, Yingpeng
Huang, Yi
Zhang, Fan
Yang, Xi
Ma, Yanfeng
Chen, Yongsheng
机构
[1] Nankai Univ, Coll Chem, Key Lab Funct Polymer Mat, Inst Polymer Chem, Tianjin 300071, Peoples R China
关键词
OXIDE; SUPERCAPACITOR; COMPOSITE; ELECTRODES; REDUCTION; FILMS;
D O I
10.1021/jp206444e
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Aiming at preventing restacking of individual graphene sheets by using a simple green hydrothermal route, we have introduced carbon nanotubes to act as the spacer in fabricating a three-dimensional (3-D) hierarchical structure with graphene sheets. These 3-D hierarchical structure materials have been used to fabricate supercapacitor devices, and a high specific capacitance of 318 F/g for graphene with an energy density of 11.1 (W h)/kg has been achieved.
引用
收藏
页码:23192 / 23197
页数:6
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[1]   Evaluation of solution-processed reduced graphene oxide films as transparent conductors [J].
Becerril, Hdctor A. ;
Mao, Jie ;
Liu, Zunfeng ;
Stoltenberg, Randall M. ;
Bao, Zhenan ;
Chen, Yongsheng .
ACS NANO, 2008, 2 (03) :463-470
[2]   An overview of graphene in energy production and storage applications [J].
Brownson, Dale A. C. ;
Kampouris, Dimitrios K. ;
Banks, Craig E. .
JOURNAL OF POWER SOURCES, 2011, 196 (11) :4873-4885
[3]   Ultracapacitors: why, how, and where is the technology [J].
Burke, A .
JOURNAL OF POWER SOURCES, 2000, 91 (01) :37-50
[4]   From Graphene to Metal Oxide Nanolamellas: A Phenomenon of Morphology Transmission [J].
Chen, Sheng ;
Zhu, Junwu ;
Wang, Xin .
ACS NANO, 2010, 4 (10) :6212-6218
[5]   Preparation of graphene by the rapid and mild thermal reduction of graphene oxide induced by microwaves [J].
Chen, Wufeng ;
Yan, Lifeng ;
Bangal, Prakriti R. .
CARBON, 2010, 48 (04) :1146-1152
[6]   Graphene and nanostructured MnO2 composite electrodes for supercapacitors [J].
Cheng, Qian ;
Tang, Jie ;
Ma, Jun ;
Zhang, Han ;
Shinya, Norio ;
Qin, Lu-Chang .
CARBON, 2011, 49 (09) :2917-2925
[7]  
Conway B.E., 1999, ELECTROCHEMICAL SUPE
[8]   Preparation of functionalized graphene sheets by a low-temperature thermal exfoliation approach and their electrochemical supercapacitive behaviors [J].
Du, Qinglai ;
Zheng, Mingbo ;
Zhang, Lifeng ;
Wang, Yongwen ;
Chen, Jinhua ;
Xue, Luping ;
Dai, Weijie ;
Ji, Guangbin ;
Cao, Jieming .
ELECTROCHIMICA ACTA, 2010, 55 (12) :3897-3903
[9]   A One-Step, Solvothermal Reduction Method for Producing Reduced Graphene Oxide Dispersions in Organic Solvents [J].
Dubin, Sergey ;
Gilje, Scott ;
Wang, Kan ;
Tung, Vincent C. ;
Cha, Kitty ;
Hall, Anthony S. ;
Farrar, Jabari ;
Varshneya, Rupal ;
Yang, Yang ;
Kaner, Richard B. .
ACS NANO, 2010, 4 (07) :3845-3852
[10]   A Three-Dimensional Carbon Nanotube/Graphene Sandwich and Its Application as Electrode in Supercapacitors [J].
Fan, Zhuangjun ;
Yan, Jun ;
Zhi, Linjie ;
Zhang, Qiang ;
Wei, Tong ;
Feng, Jing ;
Zhang, Milin ;
Qian, Weizhong ;
Wei, Fei .
ADVANCED MATERIALS, 2010, 22 (33) :3723-+