Electric field ionization of high Rydberg states of ar with sequences of identical pulses

被引:29
作者
Merkt, F
Rednall, RJ
Mackenzie, SR
Softley, TP
机构
[1] Physical and Theoretical Chemistry Laboratory, Oxford, OX1 3QZ, South Parks Road
关键词
D O I
10.1103/PhysRevLett.76.3526
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Novel field-ionization behavior of very high Rydberg states of Ar (n = 50-250) is observed using sequential pulsed electric fields. Fast autoionization acts as a filter against adiabatic field ionization near the P-2(1/2) threshold, whereas both diabatic and adiabatic field ionization occur near the P-2(3/2) threshold. Sequences of up to 9 equivalent pulses yield recurrent field ionization signals near the P-2(3/2) threshold, provided that the field returns close to zero between pulses, demonstrating a statistical redistribution of the Rydberg population amongst all states of a given Stark manifold near zero field.
引用
收藏
页码:3526 / 3529
页数:4
相关论文
共 12 条
[1]   DYNAMICS OF VERY HIGH RYDBERG STATES OF AROMATIC-MOLECULES [J].
BAHATT, D ;
EVEN, U ;
LEVINE, RD .
JOURNAL OF CHEMICAL PHYSICS, 1993, 98 (02) :1744-1747
[2]   FACTORS AFFECTING LIFETIMES AND RESOLUTION OF RYDBERG STATES OBSERVED IN ZERO-ELECTRON-KINETIC-ENERGY SPECTROSCOPY [J].
CHUPKA, WA .
JOURNAL OF CHEMICAL PHYSICS, 1993, 98 (06) :4520-4530
[3]   HYDROGEN-ATOM IN A UNIFORM ELECTRIC FIELD III [J].
DAMBURG, RJ ;
KOLOSOV, VV .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1979, 12 (16) :2637-2643
[4]  
Gallagher T. F., 1994, RYDBERG ATOMS, DOI DOI 10.1017/CBO9780511524530.021
[5]   STUDY OF RYDBERG-ATOM L-CHANGING COLLISIONS USING SELECTIVE FIELD-IONIZATION [J].
KELLERT, FG ;
JEYS, TH ;
MCMILLIAN, GB ;
SMITH, KA ;
DUNNING, FB ;
STEBBINGS, RF .
PHYSICAL REVIEW A, 1981, 23 (03) :1127-1133
[6]   MICROWAVE IONIZATION OF NA-ATOMS IN WEAK-TO-STRONG STATIC ELECTRIC-FIELDS [J].
LEE, CY ;
HETTEMA, JM ;
GALLAGHER, TF ;
CONOVER, CWS .
PHYSICAL REVIEW A, 1992, 46 (11) :7048-7052
[8]   ON THE LIFETIMES OF RYDBERG STATES PROBED BY DELAYED PULSED-FIELD IONIZATION [J].
MERKT, F ;
ZARE, RN .
JOURNAL OF CHEMICAL PHYSICS, 1994, 101 (05) :3495-3505
[9]  
MERKT F, 1995, HIGH RESOLUTION LASE
[10]   DYNAMICAL EFFECTS AT AVOIDED LEVEL-CROSSINGS - A STUDY OF THE LANDAU-ZENER EFFECT USING RYDBERG ATOMS [J].
RUBBMARK, JR ;
KASH, MM ;
LITTMAN, MG ;
KLEPPNER, D .
PHYSICAL REVIEW A, 1981, 23 (06) :3107-3117