Mechanical properties of glass forming systems

被引:10
作者
Ilyin, Valery [1 ]
Makedonska, Nataliya [1 ]
Procaccia, Itamar [1 ]
Schupper, Nurith [1 ]
机构
[1] Weizmann Inst Sci, Dept Chem Phys, IL-76100 Rehovot, Israel
来源
PHYSICAL REVIEW E | 2007年 / 76卷 / 05期
关键词
D O I
10.1103/PhysRevE.76.052401
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We address the interesting temperature range of a glass forming system where the mechanical properties are intermediate between those of a liquid and a solid. We employ an efficient Monte Carlo method to calculate the elastic moduli, and show that in this range of temperatures the moduli are finite for short times and vanish for long times, where short and long depend on the temperature. By invoking some exact results from statistical mechanics we offer an alternative method to compute shear moduli using molecular dynamics simulations, and compare those to the Monte Carlo method. The final conclusion is that these systems are not "viscous fluids" in the usual sense, as their actual time-dependence concatenates solidlike materials with varying local shear moduli.
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页数:4
相关论文
共 16 条
[1]   Direct identification of the glass transition: Growing length scale and the onset of plasticity [J].
Aharonov, E. ;
Bouchbinder, E. ;
Hentschel, H. G. E. ;
Ilyin, V. ;
Makedonska, N. ;
Procaccia, I. ;
Schupper, N. .
EPL, 2007, 77 (05)
[2]  
Allen MP, 1987, COMPUTER SIMULATIONS, DOI DOI 10.2307/2938686
[3]  
DENG D, 2007, PHILOS T R SOC LON A, V329, P549
[4]   Colloquium: The glass transition and elastic models of glass-forming liquids [J].
Dyre, Jeppe C. .
REVIEWS OF MODERN PHYSICS, 2006, 78 (03) :953-972
[5]   VISCOUS LIQUIDS AND GLASS TRANSITION - A POTENTIAL ENERGY BARRIER PICTURE [J].
GOLDSTEIN, M .
JOURNAL OF CHEMICAL PHYSICS, 1969, 51 (09) :3728-+
[6]   Geometric approach to the dynamic glass transition [J].
Grigera, TS ;
Cavagna, A ;
Giardina, I ;
Parisi, G .
PHYSICAL REVIEW LETTERS, 2002, 88 (05) :4
[7]   Statistical mechanics of the glass transition as revealed by a Voronoi tesselation [J].
Hentschel, H. G. E. ;
Ilyin, Valery ;
Makedonska, Nataliya ;
Procaccia, Itamar ;
Schupper, Nurith .
PHYSICAL REVIEW E, 2007, 75 (05)
[8]  
Landau L. D., 1958, Statistical Physics
[9]   STRAIN FLUCTUATIONS AND ELASTIC-CONSTANTS [J].
PARRINELLO, M ;
RAHMAN, A .
JOURNAL OF CHEMICAL PHYSICS, 1982, 76 (05) :2662-2666
[10]   POLYMORPHIC TRANSITIONS IN SINGLE-CRYSTALS - A NEW MOLECULAR-DYNAMICS METHOD [J].
PARRINELLO, M ;
RAHMAN, A .
JOURNAL OF APPLIED PHYSICS, 1981, 52 (12) :7182-7190