Computer simulations of supercooled liquids and glasses

被引:279
作者
Kob, W [1 ]
机构
[1] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany
关键词
D O I
10.1088/0953-8984/11/10/003
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
After a brief introduction to the dynamics of supercooled liquids, we discuss some of the advantages and drawbacks of computer simulations of such systems. Subsequently we present the results of computer simulations in which the dynamics of a fragile glass former, a binary Lennard-Jones system, is compared to that of a strong glass former, SiO2. This comparison gives evidence that the reason for the different temperature dependences of these two types of glass former lies in the transport mechanism for the particles in the vicinity of T-c, the critical temperature of mode-coupling theory. Whereas that for the fragile glass former is described very well by the ideal version of mode-coupling theory, that for the strong glass former is dominated by activated processes, in the last part of the article we review some simulations of glass formers in which the dynamics below the glass transition temperature was investigated. We show that such simulations might help to establish a connection between systems with self-generated disorder (e.g. structural glasses) and quenched disorder (e.g. spin glasses).
引用
收藏
页码:R85 / R115
页数:31
相关论文
共 249 条
  • [1] ACHENBACH M, 1996, THESIS U MAINZ
  • [2] FIELD-EFFECT ON AGING AND RELAXATION OF THE THERMOREMANENT MAGNETIZATION IN SPIN-GLASSES (LOW-FIELD REGIME)
    ALBA, M
    VINCENT, E
    HAMMANN, J
    OCIO, M
    [J]. JOURNAL OF APPLIED PHYSICS, 1987, 61 (08) : 4092 - 4094
  • [3] New results about aging in an orientational glass
    Alberici, F
    Doussineau, P
    Levelut, A
    [J]. EUROPHYSICS LETTERS, 1997, 39 (03): : 329 - 334
  • [4] PHASE TRANSITION FOR A HARD SPHERE SYSTEM
    ALDER, BJ
    WAINWRIGHT, TE
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1957, 27 (05) : 1208 - 1209
  • [5] Allen M. P., 1990, COMPUTER SIMULATION
  • [6] Fragile-glass behavior of a short-range p-spin model
    Alvarez, D
    Franz, S
    Ritort, F
    [J]. PHYSICAL REVIEW B, 1996, 54 (14): : 9756 - 9764
  • [7] Aging effects in glassy polymers: A Monte Carlo study
    Andrejew, E
    Baschnagel, J
    [J]. PHYSICA A, 1996, 233 (1-2): : 117 - 131
  • [8] Angell C.A., 1981, Adv. Chem. Phys, V48, P397, DOI [10.1002/9780470142684.ch5, DOI 10.1002/9780470142684.CH5]
  • [9] GLASS-FORMING LIQUIDS, ANOMALOUS LIQUIDS, AND POLYAMORPHISM IN LIQUIDS AND BIOPOLYMERS
    ANGELL, CA
    POOLE, PH
    SHAO, J
    [J]. NUOVO CIMENTO DELLA SOCIETA ITALIANA DI FISICA D-CONDENSED MATTER ATOMIC MOLECULAR AND CHEMICAL PHYSICS FLUIDS PLASMAS BIOPHYSICS, 1994, 16 (08): : 993 - 1025
  • [10] Angell CA, 1985, RELAXATION COMPLEX S