Low-Temperature Solution-Processed Tin Oxide as an Alternative Electron Transporting Layer for Efficient Perovskite Solar Cells

被引:1091
作者
Ke, Weijun [1 ,2 ,3 ]
Fang, Guojia [1 ]
Liu, Qin [1 ]
Xiong, Liangbin [1 ]
Qin, Pingli [1 ]
Tao, Hong [1 ]
Wang, Jing [1 ]
Lei, Hongwei [1 ]
Li, Borui [1 ]
Wan, Jiawei [1 ]
Yang, Guang [1 ]
Yan, Yanfa [2 ,3 ]
机构
[1] Wuhan Univ, Sch Phys & Technol, Key Lab Artificial Micro & Nanostruct, Minist Educ China, Wuhan 430072, Peoples R China
[2] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA
[3] Univ Toledo, Wright Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA
基金
中国国家自然科学基金;
关键词
HALIDE PEROVSKITES; GROWTH; TIO2; SNO2; DYNAMICS; FILMS;
D O I
10.1021/jacs.5b01994
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Lead halide perovskite solar cells with the high efficiencies typically use high-temperature processed TiO2 as the electron transporting layers (ETLs). Here, we demonstrate that low-temperature solution-processed nanocrystalline SnO2 can be an excellent alternative ETL material for efficient perovskite solar cells. Our best-performing planar cell using such a SnO2 ETL has achieved an average efficiency of 16.02%, obtained from efficiencies measured from both reverse and forward voltage scans. The outstanding performance of SnO2 ETLs is attributed to the excellent properties of nanocrystalline SnO2 films, such as good antireflection, suitable band edge positions, and high electron mobility. The simple low-temperature process is compatible with the roll-to-roll manufacturing of low-cost perovskite solar cells on flexible substrates.
引用
收藏
页码:6730 / 6733
页数:4
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