Experimental observation of revival structures in picosecond laser-induced alignment of I2 -: art. no. 153902

被引:374
作者
Rosca-Pruna, F [1 ]
Vrakking, MJJ [1 ]
机构
[1] FOM, Inst Atom & Mol Phys, AMOLF, NL-1098 SJ Amsterdam, Netherlands
关键词
D O I
10.1103/PhysRevLett.87.153902
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report the experimental observation of revival structures in the alignment of a ground-state rotational wave packet following nonresonant excitation of I-2 molecules by an intense picosecond laser pulse. The revivals appear at characteristic time delays following the excitation by the pump laser pulse, and show a significant narrowing of the angular distribution during a few picoseconds. The interaction with the pump laser also leads to a steady-state alignment of the molecule, due to rotational pumping.
引用
收藏
页码:153902 / 153902
页数:4
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