Studies on nonlinear dynamics and control of a tubular reactor with recycle

被引:30
作者
Antoniades, C [1 ]
Christofides, PD [1 ]
机构
[1] Univ Calif Los Angeles, Dept Chem Engn, Los Angeles, CA 90095 USA
关键词
D O I
10.1016/S0362-546X(01)00699-X
中图分类号
O29 [应用数学];
学科分类号
070104 ;
摘要
This paper presents a study on the dynamics and control of a tubular reactor with recycle loop where an exothermic reaction of the form A --> B takes place. Using a nonlinear distributed parameter model for the process which accounts for diffusion, convection and chemical reaction, and recycle loop dead-time, it is found that the use of the recycle loop reduces the maximum temperature inside the reactor, maintains the desired rate of production of the species B, and introduces a feedback mechanism into the process which renders the open-loop steady state unstable. To stabilize the process, a nonlinear output feedback controller is implemented on the process. The nonlinear controller is synthesized based on an approximate model obtained through application of Galerkin's method with approximate inertial manifolds (nonlinear Galerkin's method) to the detailed process model. The performance of the controller for different values of the recycle ratio is successfully tested through simulations and is found to be superior to the one achieved by nonlinear controllers synthesized based on approximate models obtained from linear Galerkin's method and nonlinear controllers which do not account for the presence of dead-time in the recycle loop.
引用
收藏
页码:5933 / 5944
页数:12
相关论文
共 15 条
[1]   Non-linear feedback control of parabolic partial differential difference equation systems [J].
Antoniades, C ;
Christofides, PD .
INTERNATIONAL JOURNAL OF CONTROL, 2000, 73 (17) :1572-1591
[2]   DYNAMIC PROFILES IN CHEMICAL REACTORS WITH RECYCLE [J].
BEREZOWSKI, M .
CHEMICAL ENGINEERING SCIENCE, 1993, 48 (15) :2799-2806
[3]   METHOD FOR ANALYZING GLOBAL STABILITY OF PSEUDOHOMOGENEOUS CHEMICAL REACTORS WITH RECYCLE [J].
BEREZOWSKI, M .
CHEMICAL ENGINEERING SCIENCE, 1991, 46 (07) :1781-1785
[4]   STABILIZATION OF UNSTABLE STEADY-STATES OF ADIABATIC TUBULAR REACTORS WITH RECYCLE [J].
BEREZOWSKI, M .
CHEMICAL ENGINEERING SCIENCE, 1995, 50 (12) :1989-1996
[5]   A SUFFICIENT CONDITION FOR THE EXISTENCE OF SINGLE STEADY-STATES IN CHEMICAL REACTORS WITH RECYCLE [J].
BEREZOWSKI, M .
CHEMICAL ENGINEERING SCIENCE, 1990, 45 (05) :1325-1329
[6]   Feedback control of hyperbolic PDE systems [J].
Christofides, PD ;
Daoutidis, P .
AICHE JOURNAL, 1996, 42 (11) :3063-3086
[7]   Chaotic dynamics in homogeneous tubular reactors with recycle [J].
Jacobsen, EW ;
Berezowski, M .
CHEMICAL ENGINEERING SCIENCE, 1998, 53 (23) :4023-4029
[8]   THE BIFURCATION BEHAVIOR OF TUBULAR REACTORS [J].
JENSEN, KF ;
RAY, WH .
CHEMICAL ENGINEERING SCIENCE, 1982, 37 (02) :199-222
[9]  
KARAFYLLIS I, 1997, AICHE ANN M LOS ANG
[10]  
Ray W.H., 1981, ADV PROCESS CONTROL