Study on influence of catalysts on product distribution during liquefaction of Pakistani coal

被引:22
作者
Ahmad, Imtiaz
Khan, Mohammad Arsala
Shakirullah, Mohammad
Ishaq, Mohammad
Ahmad, Rashid
Rehman, Habib Ur
Rehman, Saeed Ur
机构
[1] Univ Peshawar, Inst Chem Sci, Peshawar, Pakistan
[2] Yanbu Ind Coll, Dept Chem Engn, Yanbu Al Sinayah, Saudi Arabia
[3] Pakistan Atom Energy Commiss, Islamabad, Pakistan
关键词
coal liquefaction; synthetic fuels; catalysis; catalysts; nanostructures; pentane soluble; pentane insoluble;
D O I
10.1016/j.enconman.2007.04.015
中图分类号
O414.1 [热力学];
学科分类号
摘要
The influence of a group of metal oxide, hydroxide and chloride catalysts on the yields of liquefied products has been identified. The results of hydrogenation experiments performed with varying coal to catalyst ratio for a slurry of lignite coal in toluene demonstrated that metal loadings even as low as 1% proved effective for enhancement of yields. Among the catalysts employed, halide catalysts proved to be the most effective in terms of high yields of desirable liquefied products. (c) 2007 Elsevier Ltd. All rights reserved.
引用
收藏
页码:2502 / 2507
页数:6
相关论文
共 31 条
[1]
MECHANISM FOR COKING OF COAL-LIQUEFACTION CATALYSTS INVOLVING BASIC NITROGEN-COMPOUNDS, SODIUM AND CATALYST ACID SITES [J].
ADKINS, BD ;
MILBURN, DR ;
GOODMAN, JP ;
DAVIS, BH .
APPLIED CATALYSIS, 1988, 44 (1-2) :199-222
[2]
ANDREW P, 2004, J CHEM EDUC, V81, P673
[3]
EXFOLIATED MOS2 CATALYSTS IN COAL-LIQUEFACTION [J].
BOCKRATH, BC ;
PARFITT, DS .
CATALYSIS LETTERS, 1995, 33 (1-2) :201-207
[4]
Bönnemann H, 2001, EUR J INORG CHEM, P2455
[5]
Synthesis of open-ended MoS2 nanotubes and the application as the catalyst of methanation [J].
Chen, J ;
Li, SL ;
Xu, Q ;
Tanaka, K .
CHEMICAL COMMUNICATIONS, 2002, (16) :1722-1723
[6]
MOLYBDENUM-DISULFIDE IN THE POORLY CRYSTALLINE RAG STRUCTURE [J].
CHIANELLI, RR ;
PRESTRIDGE, EB ;
PECORARO, TA ;
DENEUFVILLE, JP .
SCIENCE, 1979, 203 (4385) :1105-1107
[7]
Ferric-sulfide-based catalysts made using reverse micelles: Effect of preparation on performance in coal liquefaction [J].
Dadyburjor, DB ;
Fout, TE ;
Zondlo, JW .
CATALYSIS TODAY, 2000, 63 (01) :33-41
[8]
DEACTIVATION OF A COAL-LIQUEFACTION CATALYST - CHARACTERIZATION BY MEASUREMENTS OF CATALYTIC ACTIVITY AND CATALYST PHYSICAL-PROPERTIES [J].
DIEZ, F ;
SAJKOWSKI, DJ ;
GATES, BC .
FUEL PROCESSING TECHNOLOGY, 1992, 31 (01) :43-53
[9]
HIGH-RATE, GAS-PHASE GROWTH OF MOS2 NESTED INORGANIC FULLERENES AND NANOTUBES [J].
FELDMAN, Y ;
WASSERMAN, E ;
SROLOVITZ, DJ ;
TENNE, R .
SCIENCE, 1995, 267 (5195) :222-225
[10]
DEPENDENCE OF COAL LIQUEFACTION BEHAVIOR ON COAL CHARACTERISTICS .1. VITRINITE-RICH SAMPLES [J].
GIVEN, PH ;
CRONAUER, DC ;
SPACKMAN, W ;
LOVELL, HL ;
DAVIS, A ;
BISWAS, B .
FUEL, 1975, 54 (01) :34-39