Seasonal and interannual variability of North American isoprene emissions as determined by formaldehyde column measurements from space

被引:103
作者
Abbot, DS
Palmer, PI
Martin, RV
Chance, KV
Jacob, DJ
Guenther, A
机构
[1] Harvard Univ, Div Engn & Appl Sci, Cambridge, MA 02138 USA
[2] Harvard Smithsonian Ctr Astrophys, Atom & Mol Phys Div, Cambridge, MA 02138 USA
[3] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA
关键词
D O I
10.1029/2003GL017336
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
[1] Formaldehyde ( HCHO) columns measured from space by solar UV backscatter allow mapping of reactive hydrocarbon emissions. The principal contributor to these emissions during the growing season is the biogenic hydrocarbon isoprene, which is of great importance for driving regional and global tropospheric chemistry. We present seven years (1995-2001) of HCHO column data for North America from the Global Ozone Monitoring Experiment (GOME), and show that the general seasonal and interannual variability of these data is consistent with knowledge of isoprene emission. There are some significant regional discrepancies with the seasonal patterns predicted from current isoprene emission models, and we suggest that these may reflect flaws in the models. The interannual variability of HCHO columns observed by GOME appears to follow the interannual variability of surface temperature, as expected from current isoprene emission models.
引用
收藏
页码:ASC5 / 1
页数:4
相关论文
共 24 条
[1]  
[Anonymous], J GEOPHYS RES
[2]   Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation [J].
Bey, I ;
Jacob, DJ ;
Yantosca, RM ;
Logan, JA ;
Field, BD ;
Fiore, AM ;
Li, QB ;
Liu, HGY ;
Mickley, LJ ;
Schultz, MG .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D19) :23073-23095
[3]  
Burrows JP, 1999, J ATMOS SCI, V56, P151, DOI 10.1175/1520-0469(1999)056<0151:TGOMEG>2.0.CO
[4]  
2
[5]   Satellite observations of formaldehyde over North America from GOME [J].
Chance, K ;
Palmer, PI ;
Spurr, RJD ;
Martin, RV ;
Kurosu, TP ;
Jacob, DJ .
GEOPHYSICAL RESEARCH LETTERS, 2000, 27 (21) :3461-3464
[6]  
Duncan B.N., 2003, J GEOPHYS RES, V108
[7]  
Geron C, 2000, TREE PHYSIOL, V20, P799
[8]   Natural emissions of non-methane volatile organic compounds; carbon monoxide, and oxides of nitrogen from North America [J].
Guenther, A ;
Geron, C ;
Pierce, T ;
Lamb, B ;
Harley, P ;
Fall, R .
ATMOSPHERIC ENVIRONMENT, 2000, 34 (12-14) :2205-2230
[9]   A GLOBAL-MODEL OF NATURAL VOLATILE ORGANIC-COMPOUND EMISSIONS [J].
GUENTHER, A ;
HEWITT, CN ;
ERICKSON, D ;
FALL, R ;
GERON, C ;
GRAEDEL, T ;
HARLEY, P ;
KLINGER, L ;
LERDAU, M ;
MCKAY, WA ;
PIERCE, T ;
SCHOLES, B ;
STEINBRECHER, R ;
TALLAMRAJU, R ;
TAYLOR, J ;
ZIMMERMAN, P .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1995, 100 (D5) :8873-8892
[10]   Isoprene emission estimates and uncertainties for the Central African EXPRESSO study domain [J].
Guenther, A ;
Baugh, B ;
Brasseur, G ;
Greenberg, J ;
Harley, P ;
Klinger, L ;
Serça, D ;
Vierling, L .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D23) :30625-30639