Reappraisal of the fossil methane budget and related emission from geologic sources

被引:163
作者
Etiope, Giuseppe [1 ]
Lassey, Keith R. [3 ]
Klusman, Ronald W. [2 ]
Boschi, Enzo [1 ]
机构
[1] Ist Nazl Geofis & Vulcanol, I-00143 Rome, Italy
[2] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA
[3] Natl Inst Water & Atmospher Res, Wellington, New Zealand
关键词
D O I
10.1029/2008GL033623
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
Converging evidence from new top-down and bottom-up estimates of fossil "radiocarbon-free" methane emissions indicates that natural geologic sources account for a substantial component of the atmospheric methane budget. Comparing emission estimates based on atmospheric (CH4)-C-14 ("radiomethane") with geologic emissions from seepage, including terrestrial macroseeps, microseepage, marine seeps, and geothermal/volcanic emissions from the Earth's crust, shows that such "geo-CH4" sources can be conservatively estimated at 53 +/- 11 Tg yr(-1) globally. This makes geo-CH4 second in importance to wetlands as a natural methane source. Such a new appraisal can easily be accommodated within the uncertainty of the global methane budget as recently compiled, and recognizes the importance of geophysical out-gassing of methane generated within the lithosphere. We propose a new coherent contemporary budget in which 30 +/- 5% (based on atmospheric radiomethane measurements) of the global source of 582 +/- 87 Tg yr(-1) has fossil origin, both natural and anthropogenic.
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页数:5
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