Discreteness effects on the front propagation in the A+B→2A reaction in 3 dimensions

被引:18
作者
Mai, J [1 ]
Sokolov, IM [1 ]
Blumen, A [1 ]
机构
[1] Univ Freiburg, D-79104 Freiburg, Germany
来源
EUROPHYSICS LETTERS | 1998年 / 44卷 / 01期
关键词
D O I
10.1209/epl/i1998-00427-7
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We consider numerically the front propagation in a three-dimensional, diffusion-controlled A + B --> 2A autocatalytic reaction. We show that the interplay between local and global ordering phenomena strongly affects the reaction kinetics, and that it leads to the breakdown of the classical continuous scheme (described by the Fisher equation) even at quite small concentrations of reactants. Discreteness aspects lead to considerable deviations of the simulated behavior of chemical fronts from the continuous scheme predictions, especially in what the fronts' structure and their propagation velocities are concerned.
引用
收藏
页码:7 / 12
页数:6
相关论文
共 21 条
  • [1] THE MACROSCOPIC LIMIT IN A STOCHASTIC REACTION-DIFFUSION PROCESS
    BREUER, HP
    HUBER, W
    PETRUCCIONE, F
    [J]. EUROPHYSICS LETTERS, 1995, 30 (02): : 69 - 74
  • [2] Shift in the velocity of a front due to a cutoff
    Brunet, E
    Derrida, B
    [J]. PHYSICAL REVIEW E, 1997, 56 (03) : 2597 - 2604
  • [3] GALFI L, 1989, PHYS REV A, V38, P1609
  • [4] GRAY P, 1990, CHEM OSCILLATIONS IN, P300
  • [5] Fluctuation effects on chemical wave fronts
    Karzazi, MA
    Lemarchand, A
    Mareschal, M
    [J]. PHYSICAL REVIEW E, 1996, 54 (05): : 4888 - 4895
  • [6] Kotomin E., 1996, COMPREHENSIVE CHEM K, V34
  • [7] KINETICS OF BIMOLECULAR REACTIONS IN CONDENSED MEDIA - CRITICAL PHENOMENA AND MICROSCOPIC SELF-ORGANISATION
    KUZOVKOV, V
    KOTOMIN, E
    [J]. REPORTS ON PROGRESS IN PHYSICS, 1988, 51 (12) : 1479 - 1523
  • [8] Fractal dimension of reaction-diffusion wave fronts
    Lemarchand, A
    Nainville, I
    Mareschal, M
    [J]. EUROPHYSICS LETTERS, 1996, 36 (03): : 227 - 231
  • [9] Microscopic simulation of a wave front: Chemically induced perturbation of particle velocity distribution
    Lemarchand, A
    Nowakowski, B
    [J]. EUROPHYSICS LETTERS, 1998, 41 (04): : 455 - 460
  • [10] MICROSCOPIC SIMULATION OF A WAVE-FRONT - FLUCTUATION EFFECTS ON PROPAGATION VELOCITY AND WIDTH
    LEMARCHAND, A
    LEMARCHAND, H
    SULPICE, E
    MARESCHAL, M
    [J]. PHYSICA A, 1992, 188 (1-3): : 277 - 283