Bimolecular recombination on carbon nanotubes

被引:7
作者
Bunning, JC [1 ]
Donovan, KJ [1 ]
Scott, K [1 ]
Somerton, M [1 ]
机构
[1] Univ London Queen Mary & Westfield Coll, Dept Phys, London E1 4NS, England
关键词
D O I
10.1103/PhysRevB.71.085412
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
By using a suspension of single-walled carbon nanotubes in an applied electric field and measuring transient photoinduced currents the problem of contacting nanotubes in charge transport studies is circumvented; basic electronic transport properties are thus studied. It is observed that the peak photocurrent excited by a mode-locked laser pulse has a sublinear dependence on light intensity. Careful measurement of these phototransients has allowed a fit of the intensity dependence of the peak photocurrent to a bimolecular recombination model developed for the one-dimensional semiconductor that the nanotubes represent. Application of the model allows the determination of some microscopic transport properties. This has been done as concentration, electric field and excitation wavelength are varied.
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页数:6
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共 15 条
[1]   STATIC POLARIZABILITIES OF SINGLE-WALL CARBON NANOTUBES [J].
BENEDICT, LX ;
LOUIE, SG ;
COHEN, ML .
PHYSICAL REVIEW B, 1995, 52 (11) :8541-8549
[2]  
BOCKRATH M, 1999, NATURE, V598, P397
[3]   Observation of transient photocurrents on suspended nanotubes [J].
Bunning, JC ;
Donovan, KJ ;
Scott, K .
JOURNAL OF APPLIED PHYSICS, 2004, 96 (07) :3939-3944
[4]   INTRINSIC PHOTOCONDUCTION IN ANTHRACENE SINGLE-CRYSTALS - ELECTRIC-FIELD DEPENDENCE OF HOLE AND ELECTRON QUANTUM YIELDS [J].
CHANCE, RR ;
BRAUN, CL .
JOURNAL OF CHEMICAL PHYSICS, 1973, 59 (05) :2269-2272
[5]   Time resolved electron motion on isolated polymer chains in solution [J].
Donovan, KJ ;
Hargrave, P ;
Scott, K ;
Somerton, M ;
Spagnoli, S .
PHYSICAL REVIEW LETTERS, 1998, 81 (17) :3731-3734
[6]   PRISMATIC GLIDE AND SLIP TRANSFER ACROSS A HIGH-ANGLE GRAIN-BOUNDARY [J].
FORWOOD, CT ;
CLAREBROUGH, LM .
PHILOSOPHICAL MAGAZINE A-PHYSICS OF CONDENSED MATTER STRUCTURE DEFECTS AND MECHANICAL PROPERTIES, 1981, 44 (01) :31-41
[7]   Extraordinary mobility in semiconducting carbon nanotubes [J].
Durkop, T ;
Getty, SA ;
Cobas, E ;
Fuhrer, MS .
NANO LETTERS, 2004, 4 (01) :35-39
[8]   Photoconductivity of single carbon nanotubes [J].
Freitag, M ;
Martin, Y ;
Misewich, JA ;
Martel, R ;
Avouris, PH .
NANO LETTERS, 2003, 3 (08) :1067-1071
[9]   Photoconductivity of single-wall carbon nanotube films [J].
Fujiwara, A ;
Matsuoka, Y ;
Matsuoka, Y ;
Suematsu, H ;
Ogawa, N ;
Miyano, K ;
Kataura, H ;
Maniwa, Y ;
Suzuki, S ;
Achiba, Y .
CARBON, 2004, 42 (5-6) :919-922
[10]   Photoconductivity in semiconducting single-walled carbon nanotubes [J].
Fujiwara, A ;
Matsuoka, Y ;
Suematsu, H ;
Ogawa, N ;
Miyano, K ;
Kataura, H ;
Maniwa, Y ;
Suzuki, S ;
Achiba, Y .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS, 2001, 40 (11B) :L1229-L1231