In situ characterization of ultrafast laser pulses for sum frequency surface studies

被引：14

作者：

Arnolds, H ^{[1
]}

Symonds, JPR ^{[1
]}

Zhang, VL ^{[1
]}

King, DA ^{[1
]}

机构：

[1] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England

来源：

REVIEW OF SCIENTIFIC INSTRUMENTS | 2003年 / 74卷 / 09期

关键词：

D O I：

10.1063/1.1599069

中图分类号：

TH7 [仪器、仪表];

学科分类号：

0804 ; 080401 ; 081102 ;

摘要：

Femtosecond laser pulses used for studies of metal surfaces in ultrahigh vacuum can be characterized by sum frequency generation. Deposition of an ultrathin alkali metal film enhances the surface nonlinear response by two orders of magnitude and allows the measurement of all necessary laser pulse parameters in 30 min at a repetition rate of 10 Hz. (C) 2003 American Institute of Physics.

引用

收藏

页码：3943 / 3946

页数：4

相关论文

共 15 条

[1] SFG spectroscopy of CO/Ni(111): UV pumping and the transient hot band transition of adsorbed CO [J].

Bandara, A ;

Kano, SS ;

Onda, K ;

Katano, S ;

Kubota, J ;

Domen, K ;

Hirose, C ;

Wada, A .

BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 2002, 75 (05) :1125-1132

[2] SUBPICOSECOND TRANSIENT INFRARED-SPECTROSCOPY OF ADSORBATES - VIBRATIONAL DYNAMICS OF CO/PT(111) [J].

BECKERLE, JD ;

CAVANAGH, RR ;

CASASSA, MP ;

HEILWEIL, EJ ;

STEPHENSON, JC .

JOURNAL OF CHEMICAL PHYSICS, 1991, 95 (07) :5403-5418

[3] Femtosecond surface vibrational spectroscopy of CO adsorbed on Ru(001) during desorption [J].

Bonn, M ;

Hess, C ;

Funk, S ;

Miners, JH ;

Persson, BNJ ;

Wolf, M ;

Ertl, G .

PHYSICAL REVIEW LETTERS, 2000, 84 (20) :4653-4656

[4] The dynamics of vibrational excitations on surfaces: CO on Ru(001) [J].

Bonn, M ;

Hess, C ;

Wolf, M .

JOURNAL OF CHEMICAL PHYSICS, 2001, 115 (16) :7725-7735

[5] Collective excitations of two layers of K on Ni(111) [J].

Chiarello, G ;

Cupolillo, A ;

Amoddeo, A ;

Caputi, LS ;

Papagno, L ;

Colavita, E .

PHYSICAL REVIEW B, 1997, 55 (03) :1376-1379

[6] MOLECULAR VIBRATIONAL-ENERGY RELAXATION AT A METAL-SURFACE - METHYL THIOLATE ON AG(111) [J].

HARRIS, AL ;

ROTHBERG, L ;

DUBOIS, LH ;

LEVINOS, NJ ;

DHAR, L .

PHYSICAL REVIEW LETTERS, 1990, 64 (17) :2086-2089

[7] Theory of sum frequency generation from metal surfaces [J].

Liebsch, A .

APPLIED PHYSICS B-LASERS AND OPTICS, 1999, 68 (03) :301-304

[8] Highly simplified device for ultrashort-pulse measurement [J].

O'Shea, P ;

Kimmel, M ;

Gu, X ;

Trebino, R .

OPTICS LETTERS, 2001, 26 (12) :932-934

[9] ADSORBATE VIBRATIONAL SPECTROSCOPY BY IR VISIBLE SUM-FREQUENCY GENERATION USING CLIO-FEL - CO FROM CH3OH ELECTROCHEMICAL DECOMPOSITION ON PT [J].

PEREMANS, A ;

TADJEDDINE, A ;

GUYOTSIONNEST, P ;

PRAZERES, R ;

GLOTIN, F ;

JAROSZYNSKI, D ;

BERSET, JM ;

ORTEGA, JM .

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1994, 341 (1-3) :146-151

[10] SURFACE SUM-FREQUENCY MIXING FOR AUTOCORRELATION AND CROSS-CORRELATION OF ULTRASHORT UV AND IR PULSES [J].

PLASS, W ;

ROTTKE, H ;

HEUER, W ;

EICHHORN, G ;

ZACHARIAS, H .

APPLIED PHYSICS B-PHOTOPHYSICS AND LASER CHEMISTRY, 1992, 54 (03) :199-201