Plasmonic nanoantennas: Angular scattering properties of multipole resonances in noble metal nanorods

被引:44
作者
Encina, Ezequiel R. [1 ]
Coronado, Eduardo A. [1 ]
机构
[1] Univ Nacl Cordoba, INFIQC, CLCM, Dept Fisicoquim,Fac Ciencias Quim, RA-5000 Cordoba, Argentina
关键词
D O I
10.1021/jp7120142
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The scattering properties of multipole plasmon resonances sustained by silver and gold nanorods (NRs) are investigated using classical electrodynamics DDA (discrete dipole approximation) simulations. The angular distribution of the scattered light is examined as a function of the multipole order, NR length, noble metal nature, and dielectric environment. For a given multipole order, the dependence of the differential scattering cross section on the different variables is rationalized in terms of two different contributions to the differential scattering cross sections: the resonant wavelength and the Mueller matrix element S(11). It was found that the magnitude of S(11) for a given multipole order is mainly determined by its quantum scattering yield. By comparing the scattering patterns of finite cylinders with the radiation scattered by a point light source, it was possible to characterize and gain physical insight on the different resonance modes.
引用
收藏
页码:9586 / 9594
页数:9
相关论文
共 45 条
[1]   Angular-ratiometric plasmon-resonance based light scattering for bioaffinity sensing [J].
Aslan, K ;
Holley, P ;
Davies, L ;
Lakowicz, JR ;
Geddes, CD .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (34) :12115-12121
[2]  
Bohren C. F., 1983, ABSORPTION SCATTERIN
[3]   Chemistry and properties of nanocrystals of different shapes [J].
Burda, C ;
Chen, XB ;
Narayanan, R ;
El-Sayed, MA .
CHEMICAL REVIEWS, 2005, 105 (04) :1025-1102
[4]   Computational study of fluorescence scattering by silver nanoparticles [J].
Chowdhury, Mustafa H. ;
Gray, Stephen K. ;
Pond, James ;
Geddes, Chris D. ;
Aslan, Kadir ;
Lakowicz, Joseph R. .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2007, 24 (09) :2259-2267
[5]   Surface plasmon broadening for arbitrary shape nanoparticles: A geometrical probability approach [J].
Coronado, EA ;
Schatz, GC .
JOURNAL OF CHEMICAL PHYSICS, 2003, 119 (07) :3926-3934
[6]   Gold nanoparticles: Assembly, supramolecular chemistry, quantum-size-related properties, and applications toward biology, catalysis, and nanotechnology [J].
Daniel, MC ;
Astruc, D .
CHEMICAL REVIEWS, 2004, 104 (01) :293-346
[7]  
Draine B. T., 2004, USER GUIDE DISCRETE
[9]  
Edwards D.F., 1985, Handbook of optical constants of solids
[10]   Resonance conditions for multipole plasmon excitations in noble metal nanorods [J].
Encina, Ezequiel R. ;
Coronado, Eduardo A. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2007, 111 (45) :16796-16801