Quantum quadratic Brownian oscillator model for absorption lineshapes

被引:3
作者
Barsegov, V
Chernyak, V
Mukamel, S
机构
[1] Univ Rochester, Dept Chem, Rochester, NY 14627 USA
[2] Corning Inc, Corning, NY 14831 USA
[3] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA
关键词
D O I
10.1560/HG6U-YQMP-8A3G-NERF
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The absorption lineshape of a two-level chromophore coupled quadratically to a collective Gaussian solvation coordinate with an arbitrary Brownian oscillator spectral density is calculated exactly using a path-integral representation of the dipole correlation function in Liouville space.
引用
收藏
页码:143 / 149
页数:7
相关论文
共 22 条
[1]   Electron transfer - From isolated molecules to biomolecules [J].
Bixon, M ;
Jortner, J .
ELECTRON TRANSFER-FROM ISOLATED MOLECULES TO BIOMOLECULES, PT 1, 1999, 106 :35-202
[2]  
BOLTON JR, 1991, ADV CHEM SERIES AM C, V228
[3]   Quadratic Brownian-oscillator model for solvation dynamics in optical response [J].
Chernyak, V ;
Mukamel, S .
JOURNAL OF CHEMICAL PHYSICS, 2001, 114 (23) :10430-10435
[4]   NONLINEAR SUSCEPTIBILITIES AND COHERENT AND SPONTANEOUS RAMAN-SPECTROSCOPY OF POLYATOMIC-MOLECULES IN CONDENSED PHASES [J].
DENG, ZF ;
MUKAMEL, S .
JOURNAL OF CHEMICAL PHYSICS, 1986, 85 (04) :1738-1752
[5]  
Feynman R. P., 1972, STAT MECH
[6]   THE THEORY OF A GENERAL QUANTUM SYSTEM INTERACTING WITH A LINEAR DISSIPATIVE SYSTEM [J].
FEYNMAN, RP ;
VERNON, FL .
ANNALS OF PHYSICS, 1963, 24 (01) :118-173
[7]   Importance sampling and theory of nonequilibrium solvation dynamics in water [J].
Geissler, PL ;
Chandler, D .
JOURNAL OF CHEMICAL PHYSICS, 2000, 113 (21) :9759-9765
[8]   VIBRATIONAL-RELAXATION IN THE EXCITED ELECTRONIC STATE [J].
HIZHNYAKOV, VV .
PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 1982, 114 (02) :721-730
[9]   ON THE THERMAL BROADENING OF ZERO-PHONON IMPURITY LINES IN ABSORPTION AND FLUORESCENCE-SPECTRA [J].
HSU, D ;
SKINNER, JL .
JOURNAL OF CHEMICAL PHYSICS, 1984, 81 (04) :1604-1613
[10]  
Lancaster P, 1985, THEORY MATRICES