Heterogeneous reactions on the surface of fine particles in the atmosphere

被引:24
作者
Ding, J [1 ]
Zhu, T [1 ]
机构
[1] Peking Univ, State Key Joint Lab Environm Simulat & Pollut Con, Coll Environm Sci, Beijing 100871, Peoples R China
来源
CHINESE SCIENCE BULLETIN | 2003年 / 48卷 / 21期
关键词
environmental quality; nitrogen oxides; ozone; sulfur dioxide; uptake coefficient; surface reaction probability;
D O I
10.1360/03wb0046
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Fine particles play an important role in the atmosphere. Research on heterogeneous reactions on the surface of fine particles is one of the frontier areas of atmospheric science. In this paper, physical and chemical characteristics of fine particles in the atmosphere and the interactions between trace gases and fine particles are described, methods used in heterogeneous reactions research are discussed in detail, progress in the study of heterogeneous reactions on the surface of fine particles in the atmosphere is summarized, existing important questions are pointed out and future research directions are suggested.
引用
收藏
页码:2267 / 2276
页数:10
相关论文
共 69 条
[1]   SPECTROSCOPIC STUDIES OF OXIDIZED SOOTS [J].
AKHTER, MS ;
CHUGHTAI, AR ;
SMITH, DM .
APPLIED SPECTROSCOPY, 1991, 45 (04) :653-665
[2]   Heterogeneous reaction of NO2 on hexane soot:: A Knudsen cell and FT-IR study [J].
Al-Abadleh, HA ;
Grassian, VH .
JOURNAL OF PHYSICAL CHEMISTRY A, 2000, 104 (51) :11926-11933
[3]  
BIRGIT G, 1999, J GEOPHYS RES, V104, P5507
[4]   EXPERIMENTAL-DETERMINATION OF HONO MASS ACCOMMODATION COEFFICIENTS USING 2 DIFFERENT TECHNIQUES [J].
BONGARTZ, A ;
KAMES, J ;
SCHURATH, U ;
GEORGE, C ;
MIRABEL, P ;
PONCHE, JL .
JOURNAL OF ATMOSPHERIC CHEMISTRY, 1994, 18 (02) :149-169
[5]   Heterogeneous uptake kinetics of volatile organic compounds on oxide surfaces using a Knudsen cell reactor:: Adsorption of acetic acid, formaldehyde, and methanol on α-Fe2O3, α-Al2O3, and SiO2 [J].
Carlos-Cuellar, S ;
Li, P ;
Christensen, AP ;
Krueger, BJ ;
Burrichter, C ;
Grassian, VH .
JOURNAL OF PHYSICAL CHEMISTRY A, 2003, 107 (21) :4250-4261
[6]   TEMPORAL AND SPATIAL VARIATIONS OF PM(2.5) AND PM(10) AEROSOL IN THE SOUTHERN CALIFORNIA AIR-QUALITY STUDY [J].
CHOW, JC ;
WATSON, JG ;
FUJITA, EM ;
LU, ZQ ;
LAWSON, DR ;
ASHBAUGH, LL .
ATMOSPHERIC ENVIRONMENT, 1994, 28 (12) :2061-2080
[7]   Uptake of gas-phase SO2 and H2O2 by ice surfaces:: Dependence on partial pressure, temperature, and surface acidity [J].
Clegg, SM ;
Abbatt, JPD .
JOURNAL OF PHYSICAL CHEMISTRY A, 2001, 105 (27) :6630-6636
[8]   ARRESTED FORMATION OF CARBON OXIDES IN PROGRAMMED OXIDATION OF METHANE ON NONSTOICHIOMETRIC SAMARIA [J].
COLUSSI, AJ ;
AMOREBIETA, VT .
JOURNAL OF PHYSICAL CHEMISTRY, 1995, 99 (38) :13921-13925
[9]  
DAVID D, 1999, J PHYS CHEM A, V103, P4865
[10]   Heterogeneous chemistry in the troposphere: experimental approaches and applications to the chemistry of sea salt particles [J].
De Haan, DO ;
Brauers, T ;
Oum, K ;
Stutz, J ;
Nordmeyer, T ;
Finlayson-Pitts, BJ .
INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY, 1999, 18 (03) :343-385