Spatial distributions and seasonal cycles of aerosols in India and China seen in global climate-aerosol model

被引:45
作者
Henriksson, S. V. [1 ]
Laaksonen, A. [1 ,2 ]
Kerminen, V. -M. [1 ]
Raisanen, P. [1 ]
Jarvinen, H. [1 ]
Sundstrom, A. -M. [3 ]
de Leeuw, G. [1 ,3 ]
机构
[1] Finnish Meteorol Inst, FIN-00101 Helsinki, Finland
[2] Univ Kuopio, Dept Appl Phys, FIN-70211 Kuopio, Finland
[3] Univ Helsinki, Dept Phys, Helsinki, Finland
基金
芬兰科学院;
关键词
SULFUR-DIOXIDE EMISSIONS; ASIAN AEROSOLS; EAST-ASIA; INVENTORY; NUCLEATION; PARAMETERS; ATMOSPHERE; IMPACT; GASES; MODIS;
D O I
10.5194/acp-11-7975-2011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A climate-aerosol model is employed to study spatial and temporal variability of aerosol properties over India and China for recent (year 2006) and future conditions (year 2020) under different emission pathways. We present results for aerosol mass concentration in different size classes and optical properties for the five different aerosol species treated by the model. Aerosol mass concentration and optical depth have significant contributions from both anthropogenic and natural aerosols. Different species have maxima in different regions, with the highest anthropogenic aerosol concentrations found in Kolkata and elsewhere in the Ganges basin in India and on the northern part of the east coast and in the Sichuan basin in China. In India, natural aerosols have a maximum in the summer due to higher wind speeds, whereas anthropogenic aerosols have a maximum in the winter due to less efficient wet removal. Surface concentrations also tend to be higher in winter due to the additional reason of lower average boundary layer height. In China, seasonal cycles are weaker with natural aerosols having a maximum in the spring and sulfate contribution to the aerosol optical depth (AOD) being higher in the latter half of the year. MODIS AOD spatial distributions are reproduced well by the model, except for the Ganges valley with high absorption and for the Thar desert with high dust concentrations. Seasonal cycles compare qualitatively well with MODIS measurements.
引用
收藏
页码:7975 / 7990
页数:16
相关论文
共 62 条
[1]   A regional scale chemical transport modeling of Asian aerosols with data assimilation of AOD observations using optimal interpolation technique [J].
Adhikary, B. ;
Kulkarni, S. ;
Dallura, A. ;
Tang, Y. ;
Chai, T. ;
Leung, L. R. ;
Qian, Y. ;
Chung, C. E. ;
Ramanathan, V. ;
Carmichael, G. R. .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (37) :8600-8615
[2]   Characterization of the seasonal cycle of south Asian aerosols: A regional-scale modeling analysis [J].
Adhikary, Bhupesh ;
Carmichael, Gregory R. ;
Tang, Youhua ;
Leung, L. Ruby ;
Qian, Yun ;
Schauer, James J. ;
Stone, Elizabeth A. ;
Ramanathan, Veerabhadran ;
Ramana, Muvva V. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2007, 112 (D22)
[3]  
Alberts B, 2008, SCIENCE, V322, P362
[4]   A time-averaged inventory of subaerial volcanic sulfur emissions [J].
Andres, RJ ;
Kasgnoc, AD .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1998, 103 (D19) :25251-25261
[5]  
[Anonymous], MAX PLANCK INSTITUT
[6]  
BALKANSKI Y, 1991, THESIS HARVARD U
[7]   Spatial distribution of aerosol black carbon over India during pre-monsoon season [J].
Beegum, S. Naseema ;
Moorthy, K. Krishna ;
Babu, S. Suresh ;
Satheesh, S. K. ;
Vinoj, V. ;
Badarinath, K. V. S. ;
Safai, P. D. ;
Devara, P. C. S. ;
Singh, Sacchidanand ;
Vinod ;
Durnka, U. C. ;
Pant, P. .
ATMOSPHERIC ENVIRONMENT, 2009, 43 (05) :1071-1078
[8]  
Bruce N., 2002, The health effects of indoor air pollution exposure in developing countries WHO/SDE/OEH/02.05
[9]   Asian Aerosols: Current and Year 2030 Distributions and Implications to Human Health and Regional Climate Change [J].
Carmichael, Gregory R. ;
Adhikary, Bhupesh ;
Kulkarni, Sarika ;
D'Allura, Alessio ;
Tang, Youhua ;
Streets, David ;
Zhang, Qiang ;
Bond, Tami C. ;
Ramanathan, Veerabhadran ;
Jamroensan, Aditsuda ;
Marrapu, Pallavi .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (15) :5811-5817
[10]   The importance of carbon and mineral dust to seasonal aerosol properties in the Nepal Himalaya [J].
Carrico, CM ;
Bergin, MH ;
Shrestha, AB ;
Dibb, JE ;
Gomes, L ;
Harris, JM .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (20) :2811-2824