Computational approaches to the determination of active site structures and reaction mechanisms in heterogeneous catalysts

被引:80
作者
Catlow, CRA
French, SA
Sokol, AA
Thomas, JM
机构
[1] Royal Inst Great Britain, Davy Faraday Res Lab, London W1S 4BS, England
[2] UCL, Dept Chem, London WC1E 6BT, England
[3] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB2 3Q2, England
来源
PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES | 2005年 / 363卷 / 1829期
基金
英国工程与自然科学研究理事会;
关键词
partial oxidation; methanol synthesis; C-H bond activation; quantum chemistry; density functional theory; embedding;
D O I
10.1098/rsta.2004.1529
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
We apply quantum chemical methods to the study of active site structures and reaction mechanisms in mesoporous silica and metal oxide catalysts. Our approach is based on the use of both molecular cluster and embedded cluster (QM/MM) techniques, where the active site and molecular complex are described using density functional theory (DFT) and the embedding matrix simulated by shell model potentials. We consider three case studies: alkene epoxidation over the microporous TS-1 catalyst; methanol synthesis on ZnO and Cu/ZnO and C-H bond activation over Li-doped MgO.
引用
收藏
页码:913 / 936
页数:24
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