Liquid holdup and pressure drop in the gas-liquid cocurrent downflow packed-bed reactor under elevated pressures

被引:17
作者
Guo, J [1 ]
Al-Dahhan, M [1 ]
机构
[1] Washington Univ, CREL, Dept Chem Engn, St Louis, MO 63130 USA
关键词
packed bed; multiphase flow; moment analysis; porous media; pressure drop; residence time distribution;
D O I
10.1016/j.ces.2004.07.106
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
An experimental investigation of the residence time distribution, liquid holdup, and pressure drop in a gas-liquid downflow packed bed reactor with porous particles operated under elevated pressures is presented. The effects of the two-phase flow rates and reactor pressures on the external liquid holdup and pressure drop are discussed. A mechanistic model, which accounts for the interaction between the gas and liquid phases by incorporating the shear and velocity slip factors between phases, is employed to predict the external liquid holdup and pressure drop for the experimentally covered flow regime. The involved parameters, such as shear and velocity slip factors and Ergun single-phase flow bed constants, are calculated from the correlations developed via neural network regression. The model's predictions and the experimental observations at elevated pressure are compared. (C) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:5387 / 5393
页数:7
相关论文
共 11 条
[1]   Prediction of pressure drop and liquid holdup in high-pressure trickle-bed reactors [J].
Al-Dahhan, MH ;
Khadilkar, MR ;
Wu, Y ;
Dudukovic, MP .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1998, 37 (03) :793-798
[2]   Pressure drop and liquid holdup in high pressure trickle-bed reactors [J].
Al-Dahhan, Muthanna H. ;
Dudukovic, Milorad P. .
CHEMICAL ENGINEERING SCIENCE, 1994, 49 (24B) :5681-5698
[3]   High-pressure trickle-bed reactors: A review [J].
AlDahhan, MH ;
Larachi, F ;
Dudukovic, MP ;
Laurent, A .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1997, 36 (08) :3292-3314
[4]   CATALYTIC REMOVAL OF PHENOL FROM AQUEOUS-PHASE USING OXYGEN OR AIR AS OXIDANT [J].
FORTUNY, A ;
FERRER, C ;
BENGOA, C ;
FONT, J ;
FABREGAT, A .
CATALYSIS TODAY, 1995, 24 (1-2) :79-83
[5]  
GUPTA P, 1999, FLOW MEASUREMENT INS, V11, P2
[6]   A PHENOMENOLOGICAL MODEL FOR PRESSURE-DROP, LIQUID HOLDUP, AND FLOW REGIME TRANSITION IN GAS-LIQUID TRICKLE FLOW [J].
HOLUB, RA ;
DUDUKOVIC, MP ;
RAMACHANDRAN, PA .
CHEMICAL ENGINEERING SCIENCE, 1992, 47 (9-11) :2343-2348
[7]   Pressure drop and liquid holdup in trickle flow reactors: Improved Ergun constants and slip correlations for the slit model [J].
Iliuta, I ;
Larachi, F ;
Grandjean, BPA .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1998, 37 (12) :4542-4550
[8]   Residence time distribution of the liquid in gas-liquid cocurrent upflow fixed-bed reactors [J].
Iliuta, I ;
Thyrion, FC ;
Muntean, O ;
Giot, M .
CHEMICAL ENGINEERING SCIENCE, 1996, 51 (20) :4579-4593
[9]   Double-slit model for partially wetted trickle flow hydrodynamics [J].
Iliuta, I ;
Larachi, F ;
Al-Dahhan, MH .
AICHE JOURNAL, 2000, 46 (03) :597-609
[10]   THE HYDRODYNAMICS OF TRICKLING FLOW IN PACKED-BEDS .2. EXPERIMENTAL-OBSERVATIONS [J].
LEVEC, J ;
SAEZ, AE ;
CARBONELL, RG .
AICHE JOURNAL, 1986, 32 (03) :369-380