Microwave-assisted NO reduction by methane over Co-ZSM-5 zeolites

被引:38
作者
Chang, YF [1 ]
Sanjurjo, A [1 ]
McCarty, JG [1 ]
Krishnan, G [1 ]
Woods, B [1 ]
Wachsman, E [1 ]
机构
[1] SRI Int, Menlo Park, CA 94025 USA
关键词
microwave; NO (nitric oxide) reduction; methane as reductant; Co-NaZSM-5; Co-HZSM-5; H-ZSM-5 zeolites as catalysts;
D O I
10.1023/A:1019059902293
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The microwave-assisted reduction of NO by methane in the presence of oxygen over Co-NaZSM-5, and H-ZSM-5 catalysts was studied. We demonstrated that microwave radiation at 2.45 GHz significantly enhances the catalytic conversion of NO to N-2. High conversions (>70%) of NO were achieved over both Co-NaZSM-5 and Co-HZSM-5 zeolite catalysts at temperatures 250-400 degrees C. Under similar conditions, thermal runs failed to show significant conversion of either NO or methane.
引用
收藏
页码:187 / 191
页数:5
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