Summary of measurement intercomparisons during TRACE-P

被引:47
作者
Eisele, FL
Mauldin, L
Cantrell, C
Zondlo, M
Apel, E
Fried, A
Walega, J
Shetter, R
Lefer, B
Flocke, F
Weinheimer, A
Avery, M
Vay, S
Sachse, G
Podolske, J
Diskin, G
Barrick, JD
Singh, HB
Brune, W
Harder, H
Martinez, M
Bandy, A
Thornton, D
Heikes, B
Kondo, Y
Riemer, D
Sandholm, S
Tan, D
Talbot, R
Dibb, J
机构
[1] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80303 USA
[2] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA
[3] NASA, Langley Res Ctr, Hampton, VA 23681 USA
[4] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA
[5] Penn State Univ, Dept Meteorol, University Pk, PA 16802 USA
[6] Drexel Univ, Dept Chem, Philadelphia, PA 19104 USA
[7] Univ Rhode Isl, Grad Sch Oceanog, Narragansett, RI 02882 USA
[8] Univ Tokyo, Adv Sci & Technol Res Ctr, Meguro Ku, Tokyo 1538904, Japan
[9] Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, Miami, FL 33149 USA
[10] Univ New Hampshire, Climate Change Res Ctr, Durham, NH 03824 USA
关键词
aircraft measurement intercomparison; chemistry instruments;
D O I
10.1029/2002JD003167
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
[1] The NASA DC-8 and P-3B aircraft flew within about a kilometer or less of each other on three occasions during the Transport and Chemical Evolution Over the Pacific (TRACE-P) campaign in order to intercompare similar measurements on the two aircraft. The first and last intercomparisons were in relatively remote marine environments during transits to and from Asia. The first began with a boundary layer measurement followed by an ascent to 3 km. The second set of intercomparisons was at a fixed altitude of about 5.2 km off the coast of Japan, also in relatively clean air. Finally, the third measurement began at 5.3 km and then descended into the boundary layer. A number of measurements were compared with the best agreement observed for the most abundant compounds such as CO2 and CH4 and with very good agreement for CO, O-3, and j values. Other comparisons, including measurements of the same compounds on both aircraft and measurements of the same compound by two different instruments on the DC-8, varied over a wide range from quite good for PAN, NO, HNO3, H2O; to reasonable agreement for OH, HO2 CH2O, acetone, and methylethylketone; and to generally poor for NO2, SO2, PPN, acetaldehyde, and methanol. The comparison results, particularly those for the fast 1-s CO and O-3 measurements, suggest that credible intercomparisons can be made using two aircraft in close proximity for relatively long lifetime and stable compounds. Much new understanding can also be gained from measurements of more reactive and generally shorter lifetime compounds, but additional improvements are needed to make such studies as meaningful as those of longer lifetime compounds. Comparisons such as these, made as a component of a larger field campaign, have the advantage that they test the actual instrument configuration used during the field study and they require no additional instrument installation and testing.
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页数:20
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