Domino effects in photoinduced structural change in one-dimensional systems

被引:40
作者
Koshino, K [1 ]
Ogawa, T
机构
[1] Tohoku Univ, Dept Phys, Aoba Ku, Sendai, Miyagi 9808578, Japan
[2] Univ Tokyo, Inst Phys, Tokyo 1538902, Japan
关键词
photoinduced structural change; cooperative transition; metastability; adiabatic approximation; lattice relaxation; domino effect;
D O I
10.1143/JPSJ.67.2174
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The possibility of occurrence of cooperative structural changes is investigated using a minimal model composed of localized electrons and classical lattices under the adiabatic approximation. In particular, the relaxation after one-photon absorption at a site is examined in detail. This relaxation proceeds in two steps. First, a local structural change is created due to the lattice relaxation associated with the local electronic excitation. After the spontaneous emission of a photon, this local structural change (a) remains locally, (b) induces a global structural change cooperatively, or (c) disappears and returns to the initial phase. Dynamical features of the case (b) are shown to be characterized by the domino effect, This global structural change occurs only when the intersite interaction is short-ranged and moderately strong.
引用
收藏
页码:2174 / 2177
页数:4
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