Development and laboratory performance evaluation of a personal multipollutant sampler for simultaneous measurements of particulate and gaseous pollutants

被引:82
作者
Demokritou, P [1 ]
Kavouras, IG [1 ]
Ferguson, ST [1 ]
Koutrakis, P [1 ]
机构
[1] Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Environm Sci & Engn Program, Boston, MA 02115 USA
关键词
D O I
10.1080/02786820152546789
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A personal multipollutant sampler has been developed. This sampler can be used for measuring exposures to particulate matter and criteria gases. The system uses a single personal sampling pump that operates at a flow rate of 5.2 l/min. The basic unit consists of two impaction-based samplers for PM2.5 and PM10 attached to a single elutriator. Two mini PM2.5 samplers are also attached to the elutriator for organic carbon (OC), elemental carbon (EC), sulfate, and nitrate measurements. For the collection of nitrate and sulfate, the minisampler includes a miniaturized honeycomb glass denuder that is placed upstream of the filter to remove nitric acid and sulfur dioxide and to minimize artifacts. Two passive samplers can also be attached to the elutriator for measurements of gaseous copollutants such as O-3, SO2, and NO2. The performance of the multipollutant sampler was examined through a series of laboratory chamber tests. The results showed a good agreement between the multipollutant sampler and the reference methods. The overall sampler performance demonstrates its suitability for personal exposure assessment studies.
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收藏
页码:741 / 752
页数:12
相关论文
共 29 条
[1]  
BAHADORI T, 1998, THESIS HARVARD SCH P
[2]  
CHOW JC, 1992, ATMOS ENVIRON, V27, P1185
[3]  
CLAYTON CA, 1993, J EXPO ANAL ENV EPID, V3, P227
[4]  
DELAMORA JF, 1990, J AEROSOL SCI, V21, P169
[5]   Development and evaluation of an impactor for a PM2.5 speciation sampler [J].
Demokritou, P ;
Kavouras, IG ;
Harrison, D ;
Koutrakis, P .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 2001, 51 (04) :514-523
[6]   AN ASSOCIATION BETWEEN AIR-POLLUTION AND MORTALITY IN 6 UNITED-STATES CITIES [J].
DOCKERY, DW ;
POPE, CA ;
XU, XP ;
SPENGLER, JD ;
WARE, JH ;
FAY, ME ;
FERRIS, BG ;
SPEIZER, FE .
NEW ENGLAND JOURNAL OF MEDICINE, 1993, 329 (24) :1753-1759
[7]   ACUTE RESPIRATORY EFFECTS OF PARTICULATE AIR-POLLUTION [J].
DOCKERY, DW ;
POPE, CA .
ANNUAL REVIEW OF PUBLIC HEALTH, 1994, 15 :107-132
[8]  
Hinds W.C., 1982, Aerosol Technology
[9]   A CYCLONE FOR SIZE-SELECTIVE SAMPLING OF AMBIENT AIR [J].
JOHN, W ;
REISCHL, G .
JOURNAL OF THE AIR POLLUTION CONTROL ASSOCIATION, 1980, 30 (08) :872-876
[10]   MEASUREMENT OF AMBIENT OZONE USING A NITRITE-COATED FILTER [J].
KOUTRAKIS, P ;
WOLFSON, JM ;
BUNYAVIROCH, A ;
FROEHLICH, SE ;
HIRANO, K ;
MULIK, JD .
ANALYTICAL CHEMISTRY, 1993, 65 (03) :209-214