SO2 and NOx removal by electron beam and electrical discharge induced non-thermal plasmas

被引:48
作者
Ighigeanu, D
Martin, D
Zissulescu, E
Macarie, R
Oproiu, C
Cirstea, E
Iovu, H
Calinescu, I
Iacob, N
机构
[1] Natl Inst Lasers Plasma & Radiat Phys, Magurele 077125, Jud Ilfov, Romania
[2] ICPET, Environm Protect Div, Bucharest, Romania
[3] Univ Bucharest, R-71102 Bucharest, Romania
关键词
electron beam; microwave; DC and pulse discharge; SO2 and NOx removal;
D O I
10.1016/j.vacuum.2004.09.009
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
An installation containing a DC negative corona discharge reactor, a pulse corona discharge reactor and a combined electron beam and microwave induced plasma reactor is presented. SO2 is removed up to 42% through spontaneous reaction with ammonia without electron beam or microwave irradiation at the temperature below 70 degrees C. For the same removal efficiency of 98% for SO2 and 80% for NOx at separate EB irradiation of 40 kGy, the required absorbed dose is about two times smaller for simultaneous electron beam and microwave irradiation. The SO2 removal efficiency of simultaneous DC or positive discharge and microwave discharge is higher than separate DC, pulse and MW discharge. Also, the applied voltage level at which the removal efficiency reaches the maximum value is less than for the separate application of DC or pulse discharge. The NO, removal efficiency of DC or pulse discharge suffers little change by additional use of the microwave energy. (c) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:493 / 500
页数:8
相关论文
共 7 条
[1]  
Chang J. -S., 1993, NATO ASI SERIES A, V34, P1
[2]   Preliminary pilot plant tests of a corona discharge-electron beam hybrid combustion flue gas cleaning system [J].
Chang, JS ;
Looy, PC ;
Nagai, K ;
Yoshioka, T ;
Aoki, S ;
Maezawa, A .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 1996, 32 (01) :131-137
[3]  
CHANG JS, 1991, IEEE T PLASMA SCI, V19, P1151
[4]  
CIVITANO L, 1992, PLASMA TECHNOLOGY, P153
[5]   Air pollution control by electrical discharges [J].
Hackam, R ;
Akiyama, H .
IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION, 2000, 7 (05) :654-683
[6]   Removal of volatile organic compounds from air streams and industrial flue gases by non-thermal plasma technology [J].
Urashima, K ;
Chang, JS .
IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION, 2000, 7 (05) :602-614
[7]  
WLLIBALD U, 1990, RADIAT PHYS CHEM, V35, P422