Chemical composition of rainwater in the northeastern Romania, Iasi region (2003-2006)

被引:64
作者
Arsene, Cecilia [1 ]
Olarlu, Romeo Lulian [1 ]
Mihalopoulos, Nikolaos [2 ]
机构
[1] Alexandru Ioan Cuza Univ, Fac Chem, Dept Inorgan & Analyt Chem, Iasi 700506, Romania
[2] Univ Crete, Environm Chem Proc Lab, Dept Chem, Iraklion 71003, Greece
关键词
rainwater; ionic composition; deposition flux; Romania;
D O I
10.1016/j.atmosenv.2007.08.046
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Chemical composition of rainwater was studied in the northeastern Romania, Iasi region, and the concentrations of major inorganic and organic ions were measured in samples collected between April 2003 and December 2006. The pH of the rainwater is 5.92 (volume weighted mean average, VWM) suggesting a sufficient load of alkaline components neutralizing its acidity. On average, 97% of the acidity in the collected samples is neutralized by CaCO3 and NH3. Clear seasonal variations were observed for some of the identified ions (e.g. SO42-, NO3-, Ca2+, NH4+). The data obtained this work revealed that both concentrations and fluxes of anthropogenic source-related ions (e.g. SO42-, NO3- and NH4+) are among the highest reported for European sites. It is shown that meteorology and long-range transport processes may concur to their high levels. (C) 2007 Elsevier Ltd. All rights reserved.
引用
收藏
页码:9452 / 9467
页数:16
相关论文
共 23 条
[1]   Assessing decadal changes in rainwater alkalinity at a rural Mediterranean site in the Montseny Mountains (NE Spain) [J].
Avila, A ;
Rodà, F .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (17) :2881-2890
[2]   Chemical composition of size-resolved atmospheric aerosols in the eastern Mediterranean during summer and winter [J].
Bardouki, H ;
Liakakou, H ;
Economou, C ;
Sciare, J ;
Smolík, J ;
Zdímal, V ;
Eleftheriadis, K ;
Lazaridis, M ;
Dye, C ;
Mihalopoulos, N .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (02) :195-208
[3]   Aerosol, precipitation and cloud water chemistry observations on the Czech Krusne Hory plateau adjacent to a heavily industrialised valley [J].
Bridges, KS ;
Jickells, TD ;
Davies, TD ;
Zeman, Z ;
Hunova, I .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (02) :353-360
[4]   Acid Rain 2000±1000 [J].
Brimblecombe, P .
WATER AIR AND SOIL POLLUTION, 2001, 130 (1-4) :25-30
[5]   Air pollution, precipitation chemistry and forest health in the Retezat Mountains, Southern Carpathians, Romania [J].
Bytnerowicz, A ;
Badea, O ;
Popescu, F ;
Musselman, R ;
Tanase, M ;
Barbu, L ;
Fraczek, W ;
Gembasu, N ;
Surdu, A ;
Danescu, F ;
Postelnicu, D ;
Cenusa, R ;
Vasile, C .
ENVIRONMENTAL POLLUTION, 2005, 137 (03) :546-567
[6]  
Draxler R.R., 2010, HYSPLIT HYBRID SINGL
[7]   Formaldehyde in the rainwater in the eastern Mediterranean: occurrence, deposition and contribution to organic carbon budget [J].
Economou, C ;
Mihalopoulos, N .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (08) :1337-1347
[8]   Origin of observed acidic-alkaline rains in a wet-only precipitation study in a Mediterranean coastal site, Patras, Greece [J].
Glavas, S ;
Moschonas, N .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (19) :3089-3099
[9]   Long-term changes of particulate emission in the industrial region of upper Silesia (Poland) and their effect on the acidity of rainwater [J].
Hlawiczka, S ;
Dyduch, B ;
Fudala, J .
WATER AIR AND SOIL POLLUTION, 2003, 142 (1-4) :151-163
[10]   Ambient air quality and deposition trends at rural stations in the Czech Republic during 1993-2001 [J].
Hunová, I ;
Santroch, J ;
Ostatnická, J .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (06) :887-898