Experimental and numerical investigations of a jet mixing in a multifunctional channel reactor -: Passive and reactive systems

被引:15
作者
Bouaifi, M [1 ]
Mortensen, M
Andersson, R
Orciuch, W
Andersson, B
Chopard, F
Norén, T
机构
[1] Chalmers Univ Technol, Dept Chem Engn & Environm Sci, S-41296 Gothenburg, Sweden
[2] AlfaLaval AB, Proc Technol Div, Business Dev, Lund, Sweden
关键词
PIV; PLIF; CFD; multifunctional channel reactor; scalar mixing; fast reactions;
D O I
10.1205/026387604772992873
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Mixing of two liquids in a new multifunctional channel reactor developed by AlfaLaval has been studied both experimentally and through computational fluid dynamics (CFD). As the channels are quite narrow the Reynolds numbers are low and the bulk of the channel is within the turbulent boundary layer. This makes accurate a priori predictions of the flowfield difficult and experimental validation necessary. Particle image velocimetry (PIV) was used to measure the flowfield, whereas planar laser-induced fluorescence was used for a scalar concentration field. CFD simulations were performed with the commercial software Fluent 5.5. Different turbulence models were tested and compared with PIV The best predictions were obtained with a low Reynolds boundary layer k-epsilon turbulence model. Mixing of a passive tracer, including mean concentration and concentration variance, was calculated with the turbulent mixer model of Baldyga. A reactive system with diazo coupling between 1-naphthols, 2-naphthols and diazotized sulphanilic acid was studied both experimentally and theoretically due to its sensitivity to mixing conditions. The interpolation model of Baldyga was used to predict the evolution of the species. Good agreement was found between simulations and experiments for both the flow field and the reactive system.
引用
收藏
页码:274 / 283
页数:10
相关论文
共 17 条
[1]   Interaction between chemical reactions and mixing on various scales [J].
Baldyga, J ;
Bourne, JR ;
Hearn, SJ .
CHEMICAL ENGINEERING SCIENCE, 1997, 52 (04) :457-466
[3]   A CLOSURE-MODEL FOR HOMOGENEOUS CHEMICAL-REACTIONS [J].
BALDYGA, J .
CHEMICAL ENGINEERING SCIENCE, 1994, 49 (12) :1985-2003
[4]  
Baldyga J., 1999, TURBULENT MIXING CHE
[5]  
Bilger R. W., 1976, Prog. Energy Combust. Sci, V1, P87, DOI [10.1016/0360-1285(76)90022-8, DOI 10.1016/0360-1285(76)90022-8]
[6]   Experimental analysis of hydrodynamics in axially agitated tank [J].
Bugay, S ;
Escudié, R ;
Liné, A .
AICHE JOURNAL, 2002, 48 (03) :463-475
[7]  
DEUSCH S, 1998, THESIS ETH ZURICH
[8]   Planar laser induced fluorescence technique for measurements of concentration fields in continuous stirred tank reactors [J].
Houcine, I ;
Vivier, H ;
Plasari, E ;
David, R ;
Villermaux, J .
EXPERIMENTS IN FLUIDS, 1996, 22 (02) :95-102
[9]   PREDICTION OF LAMINARIZATION WITH A 2-EQUATION MODEL OF TURBULENCE [J].
JONES, WP ;
LAUNDER, BE .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 1972, 15 (02) :301-+
[10]  
Kader B., 1993, INT J HEAT MASS TRAN, V24, P1541, DOI DOI 10.1016/0017-9310(81)90220-9