Personal exposures to NO2 in the EXPOLIS-study:: relation to residential indoor, outdoor and workplace concentrations in Basel, Helsinki and Prague

Personal exposures, residential indoor, outdoor and workplace levels of nitrogen dioxide (NO2) were measured for 262 urban adult (25-55 years) participants in three EXPOLIS centres (Basel, Switzerland, Helsinki; Finland, and Prague; Czech Republic) using passive samplers for 48-h sampling periods during 1996-1997. The average residential outdoor and indoor NO2 levels were lowest in Helsinki (24 +/- 12 and 18 +/- 11 mug m(-3), respectively), highest in Prague (61 +/- 20 and 43 +/- 23 mug m(-3)), with Basel in between (36 +/- 13 and 27 +/- 13 mug m(-3)). Average workplace NO2 levels, however, were highest in Basel (36 +/- 24 mug m(-3)), lowest in Helsinki (27 +/- 15 mug m(-3)), with Prague in between (30 +/- 18 mug m(-3)). A time-weighted microenvironmental exposure model explained 74% of the personal NO2 exposure variation in all centres and in average 88% of the exposures. Log-linear regression models, using residential outdoor measurements (fixed site monitoring) combined with;residential and work characteristics (i.e. work location, using gas appliances and keeping windows open), explained 48% (37%) of the personal NO2 exposure variation. Regression models based on ambient fixed site concentrations alone explained only 11-19% of personal NO2 exposure variation. Thus, ambient fixed site monitoring alone was a poor predictor for personal NO2 exposure variation, but adding personal questionnaire information can significantly improve the predicting power. (C) 2001 Elsevier Science Ltd. All rights reserved.