Controlling continuum harmonic generation with attosecond pulses

被引:11
作者
Bandrauk, AD [1 ]
Chelkowski, S [1 ]
Nguyen, HS [1 ]
机构
[1] Univ Sherbrooke, Fac Sci, Chim Theor Lab, Sherbrooke, PQ J1K 2R1, Canada
来源
APPLIED PHYSICS B-LASERS AND OPTICS | 2003年 / 77卷 / 2-3期
关键词
Laser Pulse; Molecular System; Harmonic Generation; Intense Laser; Ionization Model;
D O I
10.1007/s00340-003-1194-7
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Photo-ionization and high-order harmonic generation (HOHG) in molecular systems under the combined action of infrared femtosecond (fs) and UV attosecond (as) intense laser pulses are investigated numerically for a one-dimensional non-Born-Oppenheimer H-2(+) ion. It is shown that such a coherent control scheme of fs-as ionization leads to significant enhancement of HOHG, with efficiencies exceeding the one obtained from a single fs pulse by several orders of magnitude. The basic mechanism for this enhancement is established as enhanced ionization and control of the recollision of a high-energy non-zero-velocity ionized electron, as compared to tunneling ionization models where the ionized electron has initial zero velocity. The combined superposition of fs-as pulses results in broad HOHG spectra with a large continuum near the cutoff, thus providing a new source for synthesizing new X-ray (vacuum ultraviolet) as pulses.
引用
收藏
页码:337 / 342
页数:6
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