Influence of residential wood combustion on local air quality

被引:81
作者
Hellen, H. [1 ]
Hakola, H. [1 ]
Haaparanta, S. [1 ]
Pietarila, H. [1 ]
Kauhaniemi, M. [1 ]
机构
[1] Finnish Meteorol Inst, FIN-00101 Helsinki, Finland
关键词
wood combustion; air quality; VOCs; PAHs; CMB;
D O I
10.1016/j.scitotenv.2008.01.019
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The importance of wood combustion to local air quality was estimated by measuring different air pollutants and conducting chemical mass balance modelling. PM10, PM2.5, PAHs and VOC concentrations in ambient air were measured in a typical Finnish residential area. Measurements were conducted in January-March 2006. For some compounds, wood combustion was clearly the main local source at this site. The effect of wood combustion was more clearly seen for organic compounds than for fine particle mass. For fine particles, background concentrations dominated. However, very high, short-lived concentration peaks were detected, when the wind direction and other weather conditions were favourable. For organic compounds, the effect of wood combustion was seen in diurnal and in two-week average concentrations. PAH-concentrations were often several times higher at the residential area than in the background. Benzene concentrations showed similar diurnal pattern as the use of wood and benzene/toluene ratios indicated that wood combustion is the most important source. A chemical mass balance model was used for studying the effect of wood combustion on the measured concentrations of VOCs. Model results showed that the main local sources for VOCs at Kurkimaki are wood combustion and traffic. Wood combustion was clearly the most important source for many compounds (e.g., benzene). (C) 2008 Elsevier B.V. All rights reserved.
引用
收藏
页码:283 / 290
页数:8
相关论文
共 28 条
[1]  
[Anonymous], 12341 EN
[2]  
[Anonymous], 2003, HLTH ASP AIR POLL PA
[3]  
[Anonymous], 2000, 12884 ISO
[4]  
[Anonymous], 1998, 18082D1 DES RES I
[5]   Analysis of methyl tert-butyl ether in the atmosphere and implications as an exclusive indicator of automobile exhaust [J].
Chang, CC ;
Lo, SJ ;
Lo, JG ;
Wang, JL .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (34) :4747-4755
[6]  
Finlayson-Pitts B. J., 2000, Chemistry of the Upper and Lower Atmosphere
[7]   Impact of wood combustion on particle levels in a residential area in Denmark [J].
Glasius, M. ;
Ketzel, M. ;
Wahlin, P. ;
Jensen, B. ;
Monster, J. ;
Berkowicz, R. ;
Palmgren, F. .
ATMOSPHERIC ENVIRONMENT, 2006, 40 (37) :7115-7124
[8]  
HAAPARANTA S, 2004, YMP TERV, V4, P10
[9]   Chemical and physical characterization of emissions from birch wood combustion in a wood stove [J].
Hedberg, E ;
Kristensson, A ;
Ohlsson, M ;
Johansson, C ;
Johansson, PÅ ;
Swietlicki, E ;
Vesely, V ;
Wideqvist, U ;
Westerholm, R .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (30) :4823-4837
[10]   Ambient air concentrations, source profiles, and source apportionment of 71 different C2-C10 volatile organic compounds in urban and residential areas of Finland [J].
Hellén, H ;
Hakola, H ;
Pirjola, L ;
Laurila, T ;
Pystynen, KH .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006, 40 (01) :103-108