Polarized inelastic neutron scattering of the partially ordered Tb2Sn2O7

被引:30
作者
Rule, K. C. [2 ]
Ehlers, G. [3 ]
Stewart, J. R. [4 ]
Cornelius, A. L. [5 ]
Deen, P. P. [4 ]
Qiu, Y. [1 ,6 ]
Wiebe, C. R. [7 ,8 ]
Janik, J. A. [7 ]
Zhou, H. D. [7 ]
Antonio, D. [5 ]
Woytko, B. W. [5 ]
Ruff, J. P. [9 ]
Dabkowska, H. A. [9 ]
Gaulin, B. D. [9 ]
Gardner, J. S. [1 ,10 ]
机构
[1] NIST, NCNR, Gaithersburg, MD 20899 USA
[2] Hahn Meitner Inst Berlin GmbH, D-14109 Berlin, Germany
[3] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA
[4] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France
[5] Univ Nevada, Las Vegas, NV 89154 USA
[6] Univ Maryland, College Pk, MD 20742 USA
[7] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA
[8] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA
[9] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada
[10] Indiana Univ, Bloomington, IN 47408 USA
关键词
D O I
10.1103/PhysRevB.76.212405
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present inelastic neutron scattering results on the geometrically frustrated pyrochlore Tb2Sn2O7. At high temperature T > 50 K, this system resembles the cooperative paramagnet Tb2Ti2O7, while at low temperature T similar to 60 mK, it displays remarkably different behavior. Powder neutron scattering, susceptibility, and specific heat techniques have shown that below 0.87 K Tb2Sn2O7 enters a partially ordered state that is characterized by two-sublattice ferrimagnetic long-range order which coexists with paramagnetic spin components. We show that (i) the low-temperature state produces a large internal field and collective excitations and (ii) the coexisting paramagnetic state persists down to 0.1 K, with spins fluctuating at a rate greater than 0.04 THz, resulting in a diffuse magnetic background to the diffraction patterns. A low-lying excitation at 1.2 meV partially softens as short-range correlations build up while cooling in the paramagnetic state.
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页数:4
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