Fullerene-Free Polymer Solar Cells with over 11% Efficiency and Excellent Thermal Stability

被引：1783

作者：

Zhao, Wenchao ^{[1
]}

Qian, Deping ^{[2
]}

Zhang, Shaoqing ^{[1
]}

Li, Sunsun ^{[1
]}

Inganas, Olle ^{[2
]}

Gao, Feng ^{[2
]}

Hou, Jianhui ^{[1
]}

机构：

[1] Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, State Key Lab Polymer Phys & Chem, Beijing 100190, Peoples R China

[2] Linkoping Univ, IFM, Biomol & Organ Elect, S-58183 Linkoping, Sweden

来源：

ADVANCED MATERIALS | 2016年 / 28卷 / 23期

关键词：

BUFFER LAYER; PERFORMANCE; DONOR; AGGREGATION; DESIGN; ENERGY; MORPHOLOGY; ABSORPTION; SEPARATION;

D O I：

10.1002/adma.201600281

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A nonfullerene-based polymer solar cell (PSC) that significantly outperforms fullerene-based PSCs with respect to the power-conversion efficiency is demonstrated for the first time. An efficiency of >11%, which is among the top values in the PSC field, and excellent thermal stability is obtained using PBDB-T and ITIC as donor and acceptor, respectively.

引用

页码：4734 / 4739

页数：6

共 55 条

[1] The Role of Driving Energy and Delocalized States for Charge Separation in Organic Semiconductors [J].

Bakulin, Artem A. ;

Rao, Akshay ;

Pavelyev, Vlad G. ;

van Loosdrecht, Paul H. M. ;

Pshenichnikov, Maxim S. ;

Niedzialek, Dorota ;

Cornil, Jerome ;

Beljonne, David ;

Friend, Richard H. .

SCIENCE, 2012, 335 (6074) :1340-1344

[2]

Brabec CJ, 2001, ADV FUNCT MATER, V11, P15, DOI 10.1002/1616-3028(200102)11:1<15::AID-ADFM15>3.0.CO

[3]

2-A

[4] Single-Junction Polymer Solar Cells Exceeding 10% Power Conversion Efficiency [J].

Chen, Jing-De ;

Cui, Chaohua ;

Li, Yan-Qing ;

Zhou, Lei ;

Ou, Qing-Dong ;

Li, Chi ;

Li, Yongfang ;

Tang, Jian-Xin .

ADVANCED MATERIALS, 2015, 27 (06) :1035-1041

[5] Polymer donor-polymer acceptor (all-polymer) solar cells [J].

Facchetti, Antonio .

MATERIALS TODAY, 2013, 16 (04) :123-132

[6] All-Polymer Solar Cells Based on Absorption-Complementary Polymer Donor and Acceptor with High Power Conversion Efficiency of 8.27% [J].

Gao, Liang ;

Zhang, Zhi-Guo ;

Xue, Lingwei ;

Min, Jie ;

Zhang, Jianqi ;

Wei, Zhixiang ;

Li, Yongfang .

ADVANCED MATERIALS, 2016, 28 (09) :1884-1890

[7] Observation of the subgap optical absorption in polymer-fullerene blend solar cells -: art. no. 052113 [J].

Goris, L ;

Poruba, A ;

Hod'ákova, L ;

Vanecek, M ;

Haenen, K ;

Nesládek, M ;

Wagner, P ;

Vanderzande, D ;

De Schepper, L ;

Manca, JV .

APPLIED PHYSICS LETTERS, 2006, 88 (05) :1-3

[8] Importance of the Donor:Fullerene Intermolecular Arrangement for High-Efficiency Organic Photovoltaics [J].

Graham, Kenneth R. ;

Cabanetos, Clement ;

Jahnke, Justin P. ;

Idso, Matthew N. ;

El Labban, Abdulrahman ;

Ndjawa, Guy O. Ngongang ;

Heumueller, Thomas ;

Vandewal, Koen ;

Salleo, Alberto ;

Chmelka, Bradley F. ;

Amassian, Aram ;

Beaujuge, Pierre M. ;

McGehee, Michael D. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2014, 136 (27) :9608-9618

[9] Laminated fabrication of polymeric photovoltaic diodes [J].

Granström, M ;

Petritsch, K ;

Arias, AC ;

Lux, A ;

Andersson, MR ;

Friend, RH .

NATURE, 1998, 395 (6699) :257-260

[10] EFFICIENT PHOTODIODES FROM INTERPENETRATING POLYMER NETWORKS [J].

HALLS, JJM ;

WALSH, CA ;

GREENHAM, NC ;

MARSEGLIA, EA ;

FRIEND, RH ;

MORATTI, SC ;

HOLMES, AB .

NATURE, 1995, 376 (6540) :498-500

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