Stability Assessment on a 3% Bilayer PbS/ZnO Quantum Dot Heterojunction Solar Cell

被引：347

作者：

Luther, Joseph M. ^{[1
]}

Gao, Jianbo ^{[1
,2
]}

Lloyd, Matthew T. ^{[1
]}

Semonin, Octavi E. ^{[1
,3
]}

Beard, Matthew C. ^{[1
]}

Nozik, Arthur J. ^{[1
,3
]}

机构：

[1] Natl Renewable Energy Lab, Golden, CO 80401 USA

[2] Univ Toledo, Toledo, OH 43606 USA

[3] Univ Colorado, Boulder, CO 80309 USA

来源：

ADVANCED MATERIALS | 2010年 / 22卷 / 33期

关键词：

PBSE NANOCRYSTAL SOLIDS; ELECTRICAL-PROPERTIES; AIR; PHOTOVOLTAICS;

D O I：

10.1002/adma.201001148

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We provide the first NREL-certified efficiency measurement on an all-inorganic, solution-processed, nanocrystal solar cell. The 3% efficient device is composed of ZnO nanocrystals and 1.3 eV PbS quantum dots with gold as the top contact. This configuration yields a stable device, retaining 95% of the starting efficiency after a 1000-hour light soak in air without encapsulation.

引用

收藏

页码：3704 / +

页数：5

相关论文

共 32 条

[1] PbSe Nanocrystal Excitonic Solar Cells [J].

Choi, Joshua J. ;

Lim, Yee-Fun ;

Santiago-Berrios, Mitk'El B. ;

Oh, Matthew ;

Hyun, Byung-Ryool ;

Sung, Liangfeng ;

Bartnik, Adam C. ;

Goedhart, Augusta ;

Malliaras, George G. ;

Abruna, Hector D. ;

Wise, Frank W. ;

Hanrath, Tobias .

NANO LETTERS, 2009, 9 (11) :3749-3755

[2] Characterization of organic solar cells: the importance of device layout [J].

Cravino, Antonio ;

Schilinsky, Pavel ;

Brabec, Christoph J. .

ADVANCED FUNCTIONAL MATERIALS, 2007, 17 (18) :3906-3910

[3] Ultrabright PbSe magic-sized clusters [J].

Evans, Christopher M. ;

Guo, Li ;

Peterson, Jeffrey J. ;

Maccagnano-Zacher, Sara ;

Krauss, Todd D. .

NANO LETTERS, 2008, 8 (09) :2896-2899

[4] Air-stable all-inorganic nanocrystal solar cells processed from solution [J].

Gur, I ;

Fromer, NA ;

Geier, ML ;

Alivisatos, AP .

SCIENCE, 2005, 310 (5747) :462-465

[5] Colloidal PbS nanocrystals with size-tunable near-infrared emission: Observation of post-synthesis self-narrowing of the particle size distribution [J].

Hines, MA ;

Scholes, GD .

ADVANCED MATERIALS, 2003, 15 (21) :1844-1849

[6] Electron Injection from Colloidal PbS Quantum Dots into Titanium Dioxide Nanoparticles [J].

Hyun, Byung-Ryool ;

Zhong, Yu-Wu. ;

Bartnik, Adam C. ;

Sun, Liangfeng ;

Abruna, Hector D. ;

Wise, Frank W. ;

Goodreau, Jason D. ;

Matthews, James R. ;

Leslie, Thomas M. ;

Borrelli, Nicholas F. .

ACS NANO, 2008, 2 (11) :2206-2212

[7] Efficient solution-processed infrared photovoltaic cells: Planarized all-inorganic bulk heterojunction devices via inter-quantum-dot bridging during growth from solution [J].

Klem, Ethan J. D. ;

MacNeil, Dean D. ;

Cyr, Paul W. ;

Levina, Larissa ;

Sargenta, Edward H. .

APPLIED PHYSICS LETTERS, 2007, 90 (18)

[8] Efficient, stable infrared photovoltaics based on solution-cast colloidal quantum dots [J].

Koleilat, Ghada I. ;

Levina, Larissa ;

Shukla, Harnik ;

Myrskog, Stefan H. ;

Hinds, Sean ;

Pattantyus-Abraham, Andras G. ;

Sargent, Edward H. .

ACS NANO, 2008, 2 (05) :833-840

[9] Ultrasensitive solution-cast quantum dot photodetectors [J].

Konstantatos, Gerasimos ;

Howard, Ian ;

Fischer, Armin ;

Hoogland, Sjoerd ;

Clifford, Jason ;

Klem, Ethan ;

Levina, Larissa ;

Sargent, Edward H. .

NATURE, 2006, 442 (7099) :180-183

[10] Quasi-seeded growth of ligand-tailored PbSe nanocrystals through cation-exchange-mediated nucleation [J].

Kovalenko, Maksym V. ;

Talapin, Dmitri V. ;

Loi, Maria Antonietta ;

Cordella, Fabrizio ;

Hesser, Guenter ;

Bodnarchuk, Maryna I. ;

Heiss, Wolfgang .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (16) :3029-3033

← 1 2 3 4 →